Magnetoelectric domain engineering from micrometer to Ångstrøm scales

The functionality of magnetoelectric multiferroics depends on the formation, size, and coupling of their magnetic and electric domains. Knowing the parameters guiding these criteria is a key effort in the emerging field of magnetoelectric domain engineering. Here we show, using a combination of piez...

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التفاصيل البيبلوغرافية
الحاوية / القاعدة:Physical Review Research
المؤلفون الرئيسيون: Marcela Giraldo, Arkadiy Simonov, Hasung Sim, Ahmed Samir Lotfy, Martin Lilienblum, Lea Forster, Elzbieta Gradauskaite, Morgan Trassin, Je-Geun Park, Thomas Lottermoser, Manfred Fiebig
التنسيق: مقال
اللغة:الإنجليزية
منشور في: American Physical Society 2024-08-01
الوصول للمادة أونلاين:http://doi.org/10.1103/PhysRevResearch.6.033139
الوصف
الملخص:The functionality of magnetoelectric multiferroics depends on the formation, size, and coupling of their magnetic and electric domains. Knowing the parameters guiding these criteria is a key effort in the emerging field of magnetoelectric domain engineering. Here we show, using a combination of piezoresponse-force microscopy, nonlinear optics, and x-ray scattering, that the correlation length setting the size of the ferroelectric domains in the multiferroic hexagonal manganites can be engineered from the micron range down to a few unit cells under the substitution of Mn^{3+} ions with Al^{3+} ions. The magnetoelectric coupling mechanism between the antiferromagnetic Mn^{3+} order and the distortive-ferroelectric order remains intact even at substantial replacement of Mn^{3+} by Al^{3+}. Hence, chemical substitution proves to be an effective tool for domain-size engineering in one of the most studied classes of multiferroics.
تدمد:2643-1564