Broadband Terahertz Spectroscopy of Phonon-Polariton Dispersion in Ferroelectrics

Electromagnetic waves at frequencies below the X-ray region strongly couple to the optical vibrational modes in a solid. These coupled excitations have been called phonon polaritons. The relationship of the polariton frequency versus the polariton wavevector shows a remarkable dispersion, especially...

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Bibliographic Details
Published in:Photonics
Main Author: Seiji Kojima
Format: Article
Language:English
Published: MDPI AG 2018-12-01
Subjects:
Online Access:https://www.mdpi.com/2304-6732/5/4/55
Description
Summary:Electromagnetic waves at frequencies below the X-ray region strongly couple to the optical vibrational modes in a solid. These coupled excitations have been called phonon polaritons. The relationship of the polariton frequency versus the polariton wavevector shows a remarkable dispersion, especially in the vicinity of the transverse and longitudinal optical mode frequencies. The significant frequency dependence enables valuable applications such as a tunable terahertz radiation source. The polariton dispersion relations of technologically important dielectric and ferroelectric crystals were reviewed in the broad terahertz range using terahertz time-domain spectroscopy, far-infrared spectroscopy, and Raman scattering spectroscopy.
ISSN:2304-6732