Anthropogenic fugitive, combustion and industrial dust is a significant, underrepresented fine particulate matter source in global atmospheric models

Global measurements of the elemental composition of fine particulate matter across several urban locations by the Surface Particulate Matter Network reveal an enhanced fraction of anthropogenic dust compared to natural dust sources, especially over Asia. We develop a global simulation of anthropogen...

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التفاصيل البيبلوغرافية
الحاوية / القاعدة:Environmental Research Letters
المؤلفون الرئيسيون: Sajeev Philip, Randall V Martin, Graydon Snider, Crystal L Weagle, Aaron van Donkelaar, Michael Brauer, Daven K Henze, Zbigniew Klimont, Chandra Venkataraman, Sarath K Guttikunda, Qiang Zhang
التنسيق: مقال
اللغة:الإنجليزية
منشور في: IOP Publishing 2017-01-01
الموضوعات:
الوصول للمادة أونلاين:https://doi.org/10.1088/1748-9326/aa65a4
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author Sajeev Philip
Randall V Martin
Graydon Snider
Crystal L Weagle
Aaron van Donkelaar
Michael Brauer
Daven K Henze
Zbigniew Klimont
Chandra Venkataraman
Sarath K Guttikunda
Qiang Zhang
author_facet Sajeev Philip
Randall V Martin
Graydon Snider
Crystal L Weagle
Aaron van Donkelaar
Michael Brauer
Daven K Henze
Zbigniew Klimont
Chandra Venkataraman
Sarath K Guttikunda
Qiang Zhang
author_sort Sajeev Philip
collection DOAJ
container_title Environmental Research Letters
description Global measurements of the elemental composition of fine particulate matter across several urban locations by the Surface Particulate Matter Network reveal an enhanced fraction of anthropogenic dust compared to natural dust sources, especially over Asia. We develop a global simulation of anthropogenic fugitive, combustion, and industrial dust which, to our knowledge, is partially missing or strongly underrepresented in global models. We estimate 2–16 μ g m ^−3 increase in fine particulate mass concentration across East and South Asia by including anthropogenic fugitive, combustion, and industrial dust emissions. A simulation including anthropogenic fugitive, combustion, and industrial dust emissions increases the correlation from 0.06 to 0.66 of simulated fine dust in comparison with Surface Particulate Matter Network measurements at 13 globally dispersed locations, and reduces the low bias by 10% in total fine particulate mass in comparison with global in situ observations. Global population-weighted PM _2.5 increases by 2.9 μ g m ^−3 (10%). Our assessment ascertains the urgent need of including this underrepresented fine anthropogenic dust source into global bottom-up emission inventories and global models.
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spelling doaj-art-c5fe3ed7aee94b0c8c4eab13761069e02025-08-19T22:01:26ZengIOP PublishingEnvironmental Research Letters1748-93262017-01-0112404401810.1088/1748-9326/aa65a4Anthropogenic fugitive, combustion and industrial dust is a significant, underrepresented fine particulate matter source in global atmospheric modelsSajeev Philip0Randall V Martin1Graydon Snider2Crystal L Weagle3Aaron van Donkelaar4Michael Brauer5Daven K Henze6Zbigniew Klimont7Chandra Venkataraman8Sarath K Guttikunda9Qiang Zhang10Department of Physics and Atmospheric Science , Dalhousie University, Halifax, Nova Scotia, Canada; Now at NASA Ames Research Center , Moffett Field, California, United States of America; Author to whom any correspondence should be addressed.Department of Physics and Atmospheric Science , Dalhousie University, Halifax, Nova Scotia, Canada; Department of Chemistry , Dalhousie University, Halifax, Nova Scotia, Canada; Harvard-Smithsonian Center for Astrophysics , Cambridge, Massachusetts, United States of America; Author to whom any correspondence should be addressed.Department of Physics and Atmospheric Science , Dalhousie University, Halifax, Nova Scotia, CanadaDepartment of Chemistry , Dalhousie University, Halifax, Nova Scotia, CanadaDepartment of Physics and Atmospheric Science , Dalhousie University, Halifax, Nova Scotia, CanadaSchool of Population and Public Health , The University of British Columbia, Vancouver, British Columbia, CanadaDepartment of Mechanical Engineering , University of Colorado at Boulder, Boulder, Colorado, United States of AmericaInternational Institute for Applied Systems Analysis , Laxenburg, AustriaDepartment of Chemical Engineering , Indian Institute of Technology Bombay, Mumbai, IndiaDivision of Atmospheric Sciences , Desert Research Institute, Reno, United States of AmericaCenter for Earth System Science , Tsinghua University, Beijing, People’s Republic of ChinaGlobal measurements of the elemental composition of fine particulate matter across several urban locations by the Surface Particulate Matter Network reveal an enhanced fraction of anthropogenic dust compared to natural dust sources, especially over Asia. We develop a global simulation of anthropogenic fugitive, combustion, and industrial dust which, to our knowledge, is partially missing or strongly underrepresented in global models. We estimate 2–16 μ g m ^−3 increase in fine particulate mass concentration across East and South Asia by including anthropogenic fugitive, combustion, and industrial dust emissions. A simulation including anthropogenic fugitive, combustion, and industrial dust emissions increases the correlation from 0.06 to 0.66 of simulated fine dust in comparison with Surface Particulate Matter Network measurements at 13 globally dispersed locations, and reduces the low bias by 10% in total fine particulate mass in comparison with global in situ observations. Global population-weighted PM _2.5 increases by 2.9 μ g m ^−3 (10%). Our assessment ascertains the urgent need of including this underrepresented fine anthropogenic dust source into global bottom-up emission inventories and global models.https://doi.org/10.1088/1748-9326/aa65a4fine particulate matteraerosoldustPM2.5fugitive dustexposure
spellingShingle Sajeev Philip
Randall V Martin
Graydon Snider
Crystal L Weagle
Aaron van Donkelaar
Michael Brauer
Daven K Henze
Zbigniew Klimont
Chandra Venkataraman
Sarath K Guttikunda
Qiang Zhang
Anthropogenic fugitive, combustion and industrial dust is a significant, underrepresented fine particulate matter source in global atmospheric models
fine particulate matter
aerosol
dust
PM2.5
fugitive dust
exposure
title Anthropogenic fugitive, combustion and industrial dust is a significant, underrepresented fine particulate matter source in global atmospheric models
title_full Anthropogenic fugitive, combustion and industrial dust is a significant, underrepresented fine particulate matter source in global atmospheric models
title_fullStr Anthropogenic fugitive, combustion and industrial dust is a significant, underrepresented fine particulate matter source in global atmospheric models
title_full_unstemmed Anthropogenic fugitive, combustion and industrial dust is a significant, underrepresented fine particulate matter source in global atmospheric models
title_short Anthropogenic fugitive, combustion and industrial dust is a significant, underrepresented fine particulate matter source in global atmospheric models
title_sort anthropogenic fugitive combustion and industrial dust is a significant underrepresented fine particulate matter source in global atmospheric models
topic fine particulate matter
aerosol
dust
PM2.5
fugitive dust
exposure
url https://doi.org/10.1088/1748-9326/aa65a4
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