Remote Density Measurements of Molten Salts via Neutron Radiography

With an increased interest in the use of molten salts in both nuclear and non-nuclear systems, measuring important thermophysical properties of specific salt mixtures becomes critical in understanding salt performance and behavior. One of the more basic and significant thermophysical properties of a...

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Published in:Journal of Imaging
Main Authors: Alexander M. Long, S. Scott Parker, D. Travis Carver, J. Matt Jackson, Marisa J. Monreal, Darcy A. Newmark, Sven C. Vogel
Format: Article
Language:English
Published: MDPI AG 2021-05-01
Subjects:
Online Access:https://www.mdpi.com/2313-433X/7/5/88
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author Alexander M. Long
S. Scott Parker
D. Travis Carver
J. Matt Jackson
Marisa J. Monreal
Darcy A. Newmark
Sven C. Vogel
author_facet Alexander M. Long
S. Scott Parker
D. Travis Carver
J. Matt Jackson
Marisa J. Monreal
Darcy A. Newmark
Sven C. Vogel
author_sort Alexander M. Long
collection DOAJ
container_title Journal of Imaging
description With an increased interest in the use of molten salts in both nuclear and non-nuclear systems, measuring important thermophysical properties of specific salt mixtures becomes critical in understanding salt performance and behavior. One of the more basic and significant thermophysical properties of a given salt system is density as a function of temperature. With this in mind, this work aims to present and layout a novel approach to measuring densities of molten salt systems using neutron radiography. This work was performed on Flight Path 5 at the Los Alamos Neutron Science Center at Los Alamos National Laboratory. In order to benchmark this initial work, three salt mixtures were measured, NaCl, LiCl (58.2 mol%) + KCl (41.8 mol%), and MgCl<inline-formula><math xmlns="http://www.w3.org/1998/Math/MathML" display="inline"><semantics><msub><mrow></mrow><mn>2</mn></msub></semantics></math></inline-formula> (32 mol%) + KCl (68 mol%). Resulting densities as a function of temperature for each sample from this work were then compared to previous works employing traditional techniques. Results from this work match well with previous literature values for all salt mixtures measured, establishing that neutron radiography is a viable technique to measure density as a function of temperature in molten salt systems. Finally, advantages of using neutron radiography over other methods are discussed and future work in improving this technique is covered.
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spelling doaj-art-e65f340b90fe4c5c81874f5a86cb033b2025-08-20T00:09:43ZengMDPI AGJournal of Imaging2313-433X2021-05-01758810.3390/jimaging7050088Remote Density Measurements of Molten Salts via Neutron RadiographyAlexander M. Long0S. Scott Parker1D. Travis Carver2J. Matt Jackson3Marisa J. Monreal4Darcy A. Newmark5Sven C. Vogel6Materials Science and Technology Division, Los Alamos National Laboratory, Los Alamos, NM 87545, USAMaterials Science and Technology Division, Los Alamos National Laboratory, Los Alamos, NM 87545, USAMaterials Science and Technology Division, Los Alamos National Laboratory, Los Alamos, NM 87545, USAMaterials Science and Technology Division, Los Alamos National Laboratory, Los Alamos, NM 87545, USAChemistry Division, Los Alamos National Laboratory, Los Alamos, NM 87545, USAPhysics Division, Los Alamos National Laboratory, Los Alamos, NM 87545, USAMaterials Science and Technology Division, Los Alamos National Laboratory, Los Alamos, NM 87545, USAWith an increased interest in the use of molten salts in both nuclear and non-nuclear systems, measuring important thermophysical properties of specific salt mixtures becomes critical in understanding salt performance and behavior. One of the more basic and significant thermophysical properties of a given salt system is density as a function of temperature. With this in mind, this work aims to present and layout a novel approach to measuring densities of molten salt systems using neutron radiography. This work was performed on Flight Path 5 at the Los Alamos Neutron Science Center at Los Alamos National Laboratory. In order to benchmark this initial work, three salt mixtures were measured, NaCl, LiCl (58.2 mol%) + KCl (41.8 mol%), and MgCl<inline-formula><math xmlns="http://www.w3.org/1998/Math/MathML" display="inline"><semantics><msub><mrow></mrow><mn>2</mn></msub></semantics></math></inline-formula> (32 mol%) + KCl (68 mol%). Resulting densities as a function of temperature for each sample from this work were then compared to previous works employing traditional techniques. Results from this work match well with previous literature values for all salt mixtures measured, establishing that neutron radiography is a viable technique to measure density as a function of temperature in molten salt systems. Finally, advantages of using neutron radiography over other methods are discussed and future work in improving this technique is covered.https://www.mdpi.com/2313-433X/7/5/88molten saltsthermophysical propertiesneutron radiography
spellingShingle Alexander M. Long
S. Scott Parker
D. Travis Carver
J. Matt Jackson
Marisa J. Monreal
Darcy A. Newmark
Sven C. Vogel
Remote Density Measurements of Molten Salts via Neutron Radiography
molten salts
thermophysical properties
neutron radiography
title Remote Density Measurements of Molten Salts via Neutron Radiography
title_full Remote Density Measurements of Molten Salts via Neutron Radiography
title_fullStr Remote Density Measurements of Molten Salts via Neutron Radiography
title_full_unstemmed Remote Density Measurements of Molten Salts via Neutron Radiography
title_short Remote Density Measurements of Molten Salts via Neutron Radiography
title_sort remote density measurements of molten salts via neutron radiography
topic molten salts
thermophysical properties
neutron radiography
url https://www.mdpi.com/2313-433X/7/5/88
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