Efficient upgrading of CO to C3 fuel using asymmetric C-C coupling active sites
Catalysts for CO electroreduction have focused on Cu, and their main products have been C2 chemicals. Here authors use the concept of asymmetric active sites to develop a class of doped Cu catalysts for C-C coupling, delivering record selectivity to n-propanol.
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| Format: | Article |
| Language: | English |
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Nature Publishing Group
2019-11-01
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| Series: | Nature Communications |
| Online Access: | https://doi.org/10.1038/s41467-019-13190-6 |
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doaj-07eb2f7d6f2847e28ba2d8860b75cb0b2021-05-11T12:17:14ZengNature Publishing GroupNature Communications2041-17232019-11-011011710.1038/s41467-019-13190-6Efficient upgrading of CO to C3 fuel using asymmetric C-C coupling active sitesXue Wang0Ziyun Wang1Tao-Tao Zhuang2Cao-Thang Dinh3Jun Li4Dae-Hyun Nam5Fengwang Li6Chun-Wei Huang7Chih-Shan Tan8Zitao Chen9Miaofang Chi10Christine M. Gabardo11Ali Seifitokaldani12Petar Todorović13Andrew Proppe14Yuanjie Pang15Ahmad R. Kirmani16Yuhang Wang17Alexander H. Ip18Lee J. Richter19Benjamin Scheffel20Aoni Xu21Shen-Chuan Lo22Shana O. Kelley23David Sinton24Edward H. Sargent25Department of Electrical and Computer Engineering, University of TorontoDepartment of Electrical and Computer Engineering, University of TorontoDepartment of Electrical and Computer Engineering, University of TorontoDepartment of Electrical and Computer Engineering, University of TorontoDepartment of Electrical and Computer Engineering, University of TorontoDepartment of Electrical and Computer Engineering, University of TorontoDepartment of Electrical and Computer Engineering, University of TorontoMaterial and Chemical Research Laboratories, Industrial Technology Research InstituteDepartment of Electrical and Computer Engineering, University of TorontoCenter for Nanophase Materials Sciences, Oak Ridge National LaboratoryCenter for Nanophase Materials Sciences, Oak Ridge National LaboratoryDepartment of Mechanical and Industrial Engineering, University of TorontoDepartment of Electrical and Computer Engineering, University of TorontoDepartment of Electrical and Computer Engineering, University of TorontoDepartment of Electrical and Computer Engineering, University of TorontoDepartment of Electrical and Computer Engineering, University of TorontoMaterials Science and Engineering Division, National Institute of Standards and Technology (NIST)Department of Electrical and Computer Engineering, University of TorontoDepartment of Electrical and Computer Engineering, University of TorontoMaterials Science and Engineering Division, National Institute of Standards and Technology (NIST)Department of Electrical and Computer Engineering, University of TorontoDepartment of Electrical and Computer Engineering, University of TorontoMaterial and Chemical Research Laboratories, Industrial Technology Research InstituteDepartment of Chemistry, University of TorontoDepartment of Mechanical and Industrial Engineering, University of TorontoDepartment of Electrical and Computer Engineering, University of TorontoCatalysts for CO electroreduction have focused on Cu, and their main products have been C2 chemicals. Here authors use the concept of asymmetric active sites to develop a class of doped Cu catalysts for C-C coupling, delivering record selectivity to n-propanol.https://doi.org/10.1038/s41467-019-13190-6 |
| collection |
DOAJ |
| language |
English |
| format |
Article |
| sources |
DOAJ |
| author |
Xue Wang Ziyun Wang Tao-Tao Zhuang Cao-Thang Dinh Jun Li Dae-Hyun Nam Fengwang Li Chun-Wei Huang Chih-Shan Tan Zitao Chen Miaofang Chi Christine M. Gabardo Ali Seifitokaldani Petar Todorović Andrew Proppe Yuanjie Pang Ahmad R. Kirmani Yuhang Wang Alexander H. Ip Lee J. Richter Benjamin Scheffel Aoni Xu Shen-Chuan Lo Shana O. Kelley David Sinton Edward H. Sargent |
| spellingShingle |
Xue Wang Ziyun Wang Tao-Tao Zhuang Cao-Thang Dinh Jun Li Dae-Hyun Nam Fengwang Li Chun-Wei Huang Chih-Shan Tan Zitao Chen Miaofang Chi Christine M. Gabardo Ali Seifitokaldani Petar Todorović Andrew Proppe Yuanjie Pang Ahmad R. Kirmani Yuhang Wang Alexander H. Ip Lee J. Richter Benjamin Scheffel Aoni Xu Shen-Chuan Lo Shana O. Kelley David Sinton Edward H. Sargent Efficient upgrading of CO to C3 fuel using asymmetric C-C coupling active sites Nature Communications |
| author_facet |
Xue Wang Ziyun Wang Tao-Tao Zhuang Cao-Thang Dinh Jun Li Dae-Hyun Nam Fengwang Li Chun-Wei Huang Chih-Shan Tan Zitao Chen Miaofang Chi Christine M. Gabardo Ali Seifitokaldani Petar Todorović Andrew Proppe Yuanjie Pang Ahmad R. Kirmani Yuhang Wang Alexander H. Ip Lee J. Richter Benjamin Scheffel Aoni Xu Shen-Chuan Lo Shana O. Kelley David Sinton Edward H. Sargent |
| author_sort |
Xue Wang |
| title |
Efficient upgrading of CO to C3 fuel using asymmetric C-C coupling active sites |
| title_short |
Efficient upgrading of CO to C3 fuel using asymmetric C-C coupling active sites |
| title_full |
Efficient upgrading of CO to C3 fuel using asymmetric C-C coupling active sites |
| title_fullStr |
Efficient upgrading of CO to C3 fuel using asymmetric C-C coupling active sites |
| title_full_unstemmed |
Efficient upgrading of CO to C3 fuel using asymmetric C-C coupling active sites |
| title_sort |
efficient upgrading of co to c3 fuel using asymmetric c-c coupling active sites |
| publisher |
Nature Publishing Group |
| series |
Nature Communications |
| issn |
2041-1723 |
| publishDate |
2019-11-01 |
| description |
Catalysts for CO electroreduction have focused on Cu, and their main products have been C2 chemicals. Here authors use the concept of asymmetric active sites to develop a class of doped Cu catalysts for C-C coupling, delivering record selectivity to n-propanol. |
| url |
https://doi.org/10.1038/s41467-019-13190-6 |
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