CO₂ geological sequestration in heterogeneous binary media: Effects of geological and operational conditions

Realistic representation of subsurface heterogeneity is essential to better understand and effectively predict the migration and trapping patterns of carbon dioxide (CO2 ) during geological carbon sequestration (GCS). Many candidate aquifers for GCS have sedimentary architectures which reflect fluvial...

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Main Authors: Reza Ershadnia, Corey D. Wallace, Mohamad Reza Soltanian
Format: Article
Language:English
Published: Yandy Scientific Press 2020-12-01
Series:Advances in Geo-Energy Research
Subjects:
Online Access:https://www.yandy-ager.com/index.php/ager/article/view/277
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spelling doaj-0b9e9044a6ba4d30b32e0078af0136c12021-01-08T02:45:32ZengYandy Scientific PressAdvances in Geo-Energy Research2208-598X2208-598X2020-12-014439240510.46690/ager.2020.04.05CO₂ geological sequestration in heterogeneous binary media: Effects of geological and operational conditionsReza Ershadnia0Corey D. Wallace1Mohamad Reza Soltanian2https://orcid.org/0000-0002-5126-0668Department of Geology, University of Cincinnati, Cincinnati, OH, USADepartment of Geology, University of Cincinnati, Cincinnati, OH, USADepartment of Geology, University of Cincinnati, Cincinnati, OH, USARealistic representation of subsurface heterogeneity is essential to better understand and effectively predict the migration and trapping patterns of carbon dioxide (CO2 ) during geological carbon sequestration (GCS). Many candidate aquifers for GCS have sedimentary architectures which reflect fluvial deposition, where coarser-grained facies with higher-permeability (e.g., sandstone) are juxtaposed within finer-grained facies with lower-permeability (e.g., shale). Because the subsurface is difficult to access and sample, geostatistical methods are often used to model the spatial distribution of geological facies across different scales. We use a transition-probability based approach to simulate heterogeneous systems with binary facies distributions and the resulting petrophysical properties at the field scale. The approach produces heterogeneity fields which honor observable and physical facies attributes (e.g., volumetric proportions, mean lengths, and juxtapositional tendencies). Further, we use the associated facies-dependent properties for both relative permeability and capillary pressure relations and their hysteretic behavior. Heterogeneous facies models are used to investigate the sensitivity of different trapping mechanisms (i.e., dissolution, residual trapping) as well as CO2 plume dynamics to variability in (1) the spatial organization and connectivity of sedimentary facies types; (2) aquifer temperature; (3) CO2 injection period; (4) perforation length; and (5) the level of impurity, represented here as methane (CH4 ) present in injected CO2 streams. Model results show that the magnitudes of residual and solubility trapping are reduced by increasing the percentage and degree of connectivity of high-permeability facies. An increase in aquifer temperature leads to a decrease in residual trapping and an increase in solubility trapping. Results also reveal that for a given volume of injected CO2 , shorter injection times yield higher total amounts of trapped CO2 . Similarly, wells perforated over a shorter thickness of the aquifer contribute to an increase in both residual and solubility trapping. We also find that increased CH4 concentrations in the injected CO2 streams decrease residual trapping while increasing solubility trapping. This effect is more pronounced at shallower depths, where the pressure and temperature of the aquifer are lower.https://www.yandy-ager.com/index.php/ager/article/view/277binary mediaaquifer heterogeneitytransition-probabilityfacies connectivityperforation lengthimpurity in co2 streaminjection periodaquifer temperature
collection DOAJ
language English
format Article
sources DOAJ
author Reza Ershadnia
Corey D. Wallace
Mohamad Reza Soltanian
spellingShingle Reza Ershadnia
Corey D. Wallace
Mohamad Reza Soltanian
CO₂ geological sequestration in heterogeneous binary media: Effects of geological and operational conditions
Advances in Geo-Energy Research
binary media
aquifer heterogeneity
transition-probability
facies connectivity
perforation length
impurity in co2 stream
injection period
aquifer temperature
author_facet Reza Ershadnia
Corey D. Wallace
Mohamad Reza Soltanian
author_sort Reza Ershadnia
title CO₂ geological sequestration in heterogeneous binary media: Effects of geological and operational conditions
title_short CO₂ geological sequestration in heterogeneous binary media: Effects of geological and operational conditions
title_full CO₂ geological sequestration in heterogeneous binary media: Effects of geological and operational conditions
title_fullStr CO₂ geological sequestration in heterogeneous binary media: Effects of geological and operational conditions
title_full_unstemmed CO₂ geological sequestration in heterogeneous binary media: Effects of geological and operational conditions
title_sort co₂ geological sequestration in heterogeneous binary media: effects of geological and operational conditions
publisher Yandy Scientific Press
series Advances in Geo-Energy Research
issn 2208-598X
2208-598X
publishDate 2020-12-01
description Realistic representation of subsurface heterogeneity is essential to better understand and effectively predict the migration and trapping patterns of carbon dioxide (CO2 ) during geological carbon sequestration (GCS). Many candidate aquifers for GCS have sedimentary architectures which reflect fluvial deposition, where coarser-grained facies with higher-permeability (e.g., sandstone) are juxtaposed within finer-grained facies with lower-permeability (e.g., shale). Because the subsurface is difficult to access and sample, geostatistical methods are often used to model the spatial distribution of geological facies across different scales. We use a transition-probability based approach to simulate heterogeneous systems with binary facies distributions and the resulting petrophysical properties at the field scale. The approach produces heterogeneity fields which honor observable and physical facies attributes (e.g., volumetric proportions, mean lengths, and juxtapositional tendencies). Further, we use the associated facies-dependent properties for both relative permeability and capillary pressure relations and their hysteretic behavior. Heterogeneous facies models are used to investigate the sensitivity of different trapping mechanisms (i.e., dissolution, residual trapping) as well as CO2 plume dynamics to variability in (1) the spatial organization and connectivity of sedimentary facies types; (2) aquifer temperature; (3) CO2 injection period; (4) perforation length; and (5) the level of impurity, represented here as methane (CH4 ) present in injected CO2 streams. Model results show that the magnitudes of residual and solubility trapping are reduced by increasing the percentage and degree of connectivity of high-permeability facies. An increase in aquifer temperature leads to a decrease in residual trapping and an increase in solubility trapping. Results also reveal that for a given volume of injected CO2 , shorter injection times yield higher total amounts of trapped CO2 . Similarly, wells perforated over a shorter thickness of the aquifer contribute to an increase in both residual and solubility trapping. We also find that increased CH4 concentrations in the injected CO2 streams decrease residual trapping while increasing solubility trapping. This effect is more pronounced at shallower depths, where the pressure and temperature of the aquifer are lower.
topic binary media
aquifer heterogeneity
transition-probability
facies connectivity
perforation length
impurity in co2 stream
injection period
aquifer temperature
url https://www.yandy-ager.com/index.php/ager/article/view/277
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