Quantitative Retrieval of Volcanic Sulphate Aerosols from IASI Observations

We developed a new retrieval algorithm based on the Infrared Atmospheric Sounding Interferometer (IASI) observations, called AEROIASI-H2SO4, to measure the extinction and mass concentration of sulphate aerosols (binary solution droplets of sulphuric acid and water), with moderate random uncertaintie...

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Main Authors: Henda Guermazi, Pasquale Sellitto, Juan Cuesta, Maxim Eremenko, Mathieu Lachatre, Sylvain Mailler, Elisa Carboni, Giuseppe Salerno, Tommaso Caltabiano, Laurent Menut, Mohamed Moncef Serbaji, Farhat Rekhiss, Bernard Legras
Format: Article
Language:English
Published: MDPI AG 2021-05-01
Series:Remote Sensing
Subjects:
Online Access:https://www.mdpi.com/2072-4292/13/9/1808
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author Henda Guermazi
Pasquale Sellitto
Juan Cuesta
Maxim Eremenko
Mathieu Lachatre
Sylvain Mailler
Elisa Carboni
Giuseppe Salerno
Tommaso Caltabiano
Laurent Menut
Mohamed Moncef Serbaji
Farhat Rekhiss
Bernard Legras
spellingShingle Henda Guermazi
Pasquale Sellitto
Juan Cuesta
Maxim Eremenko
Mathieu Lachatre
Sylvain Mailler
Elisa Carboni
Giuseppe Salerno
Tommaso Caltabiano
Laurent Menut
Mohamed Moncef Serbaji
Farhat Rekhiss
Bernard Legras
Quantitative Retrieval of Volcanic Sulphate Aerosols from IASI Observations
Remote Sensing
volcanic plumes
IASI
sulphate aerosols
inverse problems in Earth observations
author_facet Henda Guermazi
Pasquale Sellitto
Juan Cuesta
Maxim Eremenko
Mathieu Lachatre
Sylvain Mailler
Elisa Carboni
Giuseppe Salerno
Tommaso Caltabiano
Laurent Menut
Mohamed Moncef Serbaji
Farhat Rekhiss
Bernard Legras
author_sort Henda Guermazi
title Quantitative Retrieval of Volcanic Sulphate Aerosols from IASI Observations
title_short Quantitative Retrieval of Volcanic Sulphate Aerosols from IASI Observations
title_full Quantitative Retrieval of Volcanic Sulphate Aerosols from IASI Observations
title_fullStr Quantitative Retrieval of Volcanic Sulphate Aerosols from IASI Observations
title_full_unstemmed Quantitative Retrieval of Volcanic Sulphate Aerosols from IASI Observations
title_sort quantitative retrieval of volcanic sulphate aerosols from iasi observations
publisher MDPI AG
series Remote Sensing
issn 2072-4292
publishDate 2021-05-01
description We developed a new retrieval algorithm based on the Infrared Atmospheric Sounding Interferometer (IASI) observations, called AEROIASI-H2SO4, to measure the extinction and mass concentration of sulphate aerosols (binary solution droplets of sulphuric acid and water), with moderate random uncertainties (typically ∼35% total uncertainty for column mass concentration estimations). The algorithm is based on a self-adapting Tikhonov–Phillips regularization method. It is here tested over a moderate-intensity eruption of Mount Etna volcano (18 March 2012), Italy, and is used to characterise this event in terms of the spatial distribution of the retrieved plume. Comparisons with simultaneous and independent aerosol optical depth observations from MODIS (Moderate Resolution Imaging Spectroradiometer), SO<inline-formula><math xmlns="http://www.w3.org/1998/Math/MathML" display="inline"><semantics><msub><mrow></mrow><mn>2</mn></msub></semantics></math></inline-formula> plume observations from IASI and simulations with the CHIMERE chemistry/transport model show that AEROIASI-H2SO4 correctly identifies the volcanic plume horizontal morphology, thus providing crucial new information towards the study of volcanic emissions, volcanic sulphur cycle in the atmosphere, plume evolution processes, and their impacts. Insights are given on the possible spectroscopic evidence of the presence in the plume of larger-sized particles than previously reported for secondary sulphate aerosols from volcanic eruptions.
topic volcanic plumes
IASI
sulphate aerosols
inverse problems in Earth observations
url https://www.mdpi.com/2072-4292/13/9/1808
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spelling doaj-0d8f1dfb16424d2c82db74db6606838a2021-05-31T23:20:03ZengMDPI AGRemote Sensing2072-42922021-05-01131808180810.3390/rs13091808Quantitative Retrieval of Volcanic Sulphate Aerosols from IASI ObservationsHenda Guermazi0Pasquale Sellitto1Juan Cuesta2Maxim Eremenko3Mathieu Lachatre4Sylvain Mailler5Elisa Carboni6Giuseppe Salerno7Tommaso Caltabiano8Laurent Menut9Mohamed Moncef Serbaji10Farhat Rekhiss11Bernard Legras12Laboratoire Interuniversitaire des Systèmes Atmosphériques (LISA), UMR CNRS 7583, Institut Pierre Simon Laplace (IPSL), Université Paris-Est-Créteil, Université de Paris, 94000 Créteil, FranceLaboratoire Interuniversitaire des Systèmes Atmosphériques (LISA), UMR CNRS 7583, Institut Pierre Simon Laplace (IPSL), Université Paris-Est-Créteil, Université de Paris, 94000 Créteil, FranceLaboratoire Interuniversitaire des Systèmes Atmosphériques (LISA), UMR CNRS 7583, Institut Pierre Simon Laplace (IPSL), Université Paris-Est-Créteil, Université de Paris, 94000 Créteil, FranceLaboratoire Interuniversitaire des Systèmes Atmosphériques (LISA), UMR CNRS 7583, Institut Pierre Simon Laplace (IPSL), Université Paris-Est-Créteil, Université de Paris, 94000 Créteil, FranceLaboratoire de Météorologie Dynamique (LMD), UMR CNRS 8539, Ecole Polytechnique, Institut Pierre Simon Laplace, Ecole Normale Supérieure, Université Paris-Saclay, Sorbonne Universités, Route de Saclay, 91128 Palaiseau, FranceLaboratoire de Météorologie Dynamique (LMD), UMR CNRS 8539, Ecole Polytechnique, Institut Pierre Simon Laplace, Ecole Normale Supérieure, Université Paris-Saclay, Sorbonne Universités, Route de Saclay, 91128 Palaiseau, FranceCOMET, Atmospheric, Oceanic and Planetary Physics, University of Oxford, Clarendon Laboratory, Parks Road, Oxford OX1 3PU, UKIstituto Nazionale di Geofisica e Vulcanologia (INGV), OE, 95123 Catania, ItalyIstituto Nazionale di Geofisica e Vulcanologia (INGV), OE, 95123 Catania, ItalyLaboratoire de Météorologie Dynamique (LMD), UMR CNRS 8539, Ecole Polytechnique, Institut Pierre Simon Laplace, Ecole Normale Supérieure, Université Paris-Saclay, Sorbonne Universités, Route de Saclay, 91128 Palaiseau, FranceNational School of Engineers of Sfax, Water, Energy and Environment Laboratory L3E, University of Sfax, B.P 1173, 3021 Sfax, TunisiaNational School of Engineers of Sfax, Water, Energy and Environment Laboratory L3E, University of Sfax, B.P 1173, 3021 Sfax, TunisiaLaboratoire de Météorologie Dynamique (LMD), UMR CNRS 8539, Ecole Polytechnique, Institut Pierre Simon Laplace, Ecole Normale Supérieure, Université Paris-Saclay, Sorbonne Universités, Route de Saclay, 91128 Palaiseau, FranceWe developed a new retrieval algorithm based on the Infrared Atmospheric Sounding Interferometer (IASI) observations, called AEROIASI-H2SO4, to measure the extinction and mass concentration of sulphate aerosols (binary solution droplets of sulphuric acid and water), with moderate random uncertainties (typically ∼35% total uncertainty for column mass concentration estimations). The algorithm is based on a self-adapting Tikhonov–Phillips regularization method. It is here tested over a moderate-intensity eruption of Mount Etna volcano (18 March 2012), Italy, and is used to characterise this event in terms of the spatial distribution of the retrieved plume. Comparisons with simultaneous and independent aerosol optical depth observations from MODIS (Moderate Resolution Imaging Spectroradiometer), SO<inline-formula><math xmlns="http://www.w3.org/1998/Math/MathML" display="inline"><semantics><msub><mrow></mrow><mn>2</mn></msub></semantics></math></inline-formula> plume observations from IASI and simulations with the CHIMERE chemistry/transport model show that AEROIASI-H2SO4 correctly identifies the volcanic plume horizontal morphology, thus providing crucial new information towards the study of volcanic emissions, volcanic sulphur cycle in the atmosphere, plume evolution processes, and their impacts. Insights are given on the possible spectroscopic evidence of the presence in the plume of larger-sized particles than previously reported for secondary sulphate aerosols from volcanic eruptions.https://www.mdpi.com/2072-4292/13/9/1808volcanic plumesIASIsulphate aerosolsinverse problems in Earth observations