A Nanomesoporous Catalyst from Modified Red Mud and Its Application for Methane Decomposition to Hydrogen Production

A type of nanomesoporous modified red mud (MRM) catalyst was prepared and utilized for catalytic methane decomposition (CMD) to produce hydrogen. The modification process significantly simplified the mineral composition of the red mud (RM); in the meantime, the physical and chemical structure of RM...

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Main Authors: Xiaoke Fang, Quanrun Liu, Peng Li, Haipeng Li, Fenghai Li, Guangxu Huang
Format: Article
Language:English
Published: Hindawi Limited 2016-01-01
Series:Journal of Nanomaterials
Online Access:http://dx.doi.org/10.1155/2016/6947636
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spelling doaj-167fc5f25f8f4e48af2594a84d95e0a32020-11-24T21:08:37ZengHindawi LimitedJournal of Nanomaterials1687-41101687-41292016-01-01201610.1155/2016/69476366947636A Nanomesoporous Catalyst from Modified Red Mud and Its Application for Methane Decomposition to Hydrogen ProductionXiaoke Fang0Quanrun Liu1Peng Li2Haipeng Li3Fenghai Li4Guangxu Huang5School of Materials Science and Engineering, Henan Polytechnic University, Jiaozuo 454000, ChinaSchool of Materials Science and Engineering, Henan Polytechnic University, Jiaozuo 454000, ChinaSchool of Materials Science and Engineering, Henan Polytechnic University, Jiaozuo 454000, ChinaSchool of Materials Science and Engineering, Henan Polytechnic University, Jiaozuo 454000, ChinaDepartment of Chemistry and Engineering, Heze University, Heze 274000, ChinaSchool of Materials Science and Engineering, Henan Polytechnic University, Jiaozuo 454000, ChinaA type of nanomesoporous modified red mud (MRM) catalyst was prepared and utilized for catalytic methane decomposition (CMD) to produce hydrogen. The modification process significantly simplified the mineral composition of the red mud (RM); in the meantime, the physical and chemical structure of RM was changed. TEM images suggested that MRM was a kind of nanomesoporous material assembled by a number of uniformly nanoscale particles, BET results showed that the pore size distributions of MRM were ranged from 3 to 12 nm, and the specific surface area and total pore volumes of red mud improved from 8.00 m2/g and 0.08 cm3/g to 190.61 m2/g and 0.39 cm3/g, respectively. The catalytic performance of the catalysts has been tested at 800°C; the results showed that MRM exhibited much higher activity and stability than RM for CMD.http://dx.doi.org/10.1155/2016/6947636
collection DOAJ
language English
format Article
sources DOAJ
author Xiaoke Fang
Quanrun Liu
Peng Li
Haipeng Li
Fenghai Li
Guangxu Huang
spellingShingle Xiaoke Fang
Quanrun Liu
Peng Li
Haipeng Li
Fenghai Li
Guangxu Huang
A Nanomesoporous Catalyst from Modified Red Mud and Its Application for Methane Decomposition to Hydrogen Production
Journal of Nanomaterials
author_facet Xiaoke Fang
Quanrun Liu
Peng Li
Haipeng Li
Fenghai Li
Guangxu Huang
author_sort Xiaoke Fang
title A Nanomesoporous Catalyst from Modified Red Mud and Its Application for Methane Decomposition to Hydrogen Production
title_short A Nanomesoporous Catalyst from Modified Red Mud and Its Application for Methane Decomposition to Hydrogen Production
title_full A Nanomesoporous Catalyst from Modified Red Mud and Its Application for Methane Decomposition to Hydrogen Production
title_fullStr A Nanomesoporous Catalyst from Modified Red Mud and Its Application for Methane Decomposition to Hydrogen Production
title_full_unstemmed A Nanomesoporous Catalyst from Modified Red Mud and Its Application for Methane Decomposition to Hydrogen Production
title_sort nanomesoporous catalyst from modified red mud and its application for methane decomposition to hydrogen production
publisher Hindawi Limited
series Journal of Nanomaterials
issn 1687-4110
1687-4129
publishDate 2016-01-01
description A type of nanomesoporous modified red mud (MRM) catalyst was prepared and utilized for catalytic methane decomposition (CMD) to produce hydrogen. The modification process significantly simplified the mineral composition of the red mud (RM); in the meantime, the physical and chemical structure of RM was changed. TEM images suggested that MRM was a kind of nanomesoporous material assembled by a number of uniformly nanoscale particles, BET results showed that the pore size distributions of MRM were ranged from 3 to 12 nm, and the specific surface area and total pore volumes of red mud improved from 8.00 m2/g and 0.08 cm3/g to 190.61 m2/g and 0.39 cm3/g, respectively. The catalytic performance of the catalysts has been tested at 800°C; the results showed that MRM exhibited much higher activity and stability than RM for CMD.
url http://dx.doi.org/10.1155/2016/6947636
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