Polymerized small molecular acceptor based all-polymer solar cells with an efficiency of 16.16% via tuning polymer blend morphology by molecular design

Through development of non-fullerene acceptors, OPVs have reached efficiencies of 18%, yet the inadequate operational lifetime still poses a challenge for the commercialisation. Here, the authors investigate the origin of instability of NFA solar cells, and propose some strategies to mitigate this i...

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Main Authors: Jiaqi Du, Ke Hu, Jinyuan Zhang, Lei Meng, Jiling Yue, Indunil Angunawela, Hongping Yan, Shucheng Qin, Xiaolei Kong, Zhanjun Zhang, Bo Guan, Harald Ade, Yongfang Li
Format: Article
Language:English
Published: Nature Publishing Group 2021-09-01
Series:Nature Communications
Online Access:https://doi.org/10.1038/s41467-021-25638-9
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spelling doaj-17d9c97f824840eab5626fd3420daa8c2021-09-12T11:46:43ZengNature Publishing GroupNature Communications2041-17232021-09-0112111010.1038/s41467-021-25638-9Polymerized small molecular acceptor based all-polymer solar cells with an efficiency of 16.16% via tuning polymer blend morphology by molecular designJiaqi Du0Ke Hu1Jinyuan Zhang2Lei Meng3Jiling Yue4Indunil Angunawela5Hongping Yan6Shucheng Qin7Xiaolei Kong8Zhanjun Zhang9Bo Guan10Harald Ade11Yongfang Li12Beijing National Laboratory for Molecular Sciences, CAS Key Laboratory of Organic Solids, Institute of Chemistry, Chinese Academy of SciencesSchool of Chemical Science, University of Chinese Academy of SciencesBeijing National Laboratory for Molecular Sciences, CAS Key Laboratory of Organic Solids, Institute of Chemistry, Chinese Academy of SciencesBeijing National Laboratory for Molecular Sciences, CAS Key Laboratory of Organic Solids, Institute of Chemistry, Chinese Academy of SciencesCenter for Physiochemical Analysis and Measurement, Institute of Chemistry, Chinese Academy of SciencesDepartment of Physics and Organic and Carbon Electronics Lab (ORaCEL), North Carolina State UniversityDepartment of Chemical Engineering, Stanford UniversityBeijing National Laboratory for Molecular Sciences, CAS Key Laboratory of Organic Solids, Institute of Chemistry, Chinese Academy of SciencesBeijing National Laboratory for Molecular Sciences, CAS Key Laboratory of Organic Solids, Institute of Chemistry, Chinese Academy of SciencesSchool of Chemical Science, University of Chinese Academy of SciencesCenter for Physiochemical Analysis and Measurement, Institute of Chemistry, Chinese Academy of SciencesDepartment of Physics and Organic and Carbon Electronics Lab (ORaCEL), North Carolina State UniversityBeijing National Laboratory for Molecular Sciences, CAS Key Laboratory of Organic Solids, Institute of Chemistry, Chinese Academy of SciencesThrough development of non-fullerene acceptors, OPVs have reached efficiencies of 18%, yet the inadequate operational lifetime still poses a challenge for the commercialisation. Here, the authors investigate the origin of instability of NFA solar cells, and propose some strategies to mitigate this issue.https://doi.org/10.1038/s41467-021-25638-9
collection DOAJ
language English
format Article
sources DOAJ
author Jiaqi Du
Ke Hu
Jinyuan Zhang
Lei Meng
Jiling Yue
Indunil Angunawela
Hongping Yan
Shucheng Qin
Xiaolei Kong
Zhanjun Zhang
Bo Guan
Harald Ade
Yongfang Li
spellingShingle Jiaqi Du
Ke Hu
Jinyuan Zhang
Lei Meng
Jiling Yue
Indunil Angunawela
Hongping Yan
Shucheng Qin
Xiaolei Kong
Zhanjun Zhang
Bo Guan
Harald Ade
Yongfang Li
Polymerized small molecular acceptor based all-polymer solar cells with an efficiency of 16.16% via tuning polymer blend morphology by molecular design
Nature Communications
author_facet Jiaqi Du
Ke Hu
Jinyuan Zhang
Lei Meng
Jiling Yue
Indunil Angunawela
Hongping Yan
Shucheng Qin
Xiaolei Kong
Zhanjun Zhang
Bo Guan
Harald Ade
Yongfang Li
author_sort Jiaqi Du
title Polymerized small molecular acceptor based all-polymer solar cells with an efficiency of 16.16% via tuning polymer blend morphology by molecular design
title_short Polymerized small molecular acceptor based all-polymer solar cells with an efficiency of 16.16% via tuning polymer blend morphology by molecular design
title_full Polymerized small molecular acceptor based all-polymer solar cells with an efficiency of 16.16% via tuning polymer blend morphology by molecular design
title_fullStr Polymerized small molecular acceptor based all-polymer solar cells with an efficiency of 16.16% via tuning polymer blend morphology by molecular design
title_full_unstemmed Polymerized small molecular acceptor based all-polymer solar cells with an efficiency of 16.16% via tuning polymer blend morphology by molecular design
title_sort polymerized small molecular acceptor based all-polymer solar cells with an efficiency of 16.16% via tuning polymer blend morphology by molecular design
publisher Nature Publishing Group
series Nature Communications
issn 2041-1723
publishDate 2021-09-01
description Through development of non-fullerene acceptors, OPVs have reached efficiencies of 18%, yet the inadequate operational lifetime still poses a challenge for the commercialisation. Here, the authors investigate the origin of instability of NFA solar cells, and propose some strategies to mitigate this issue.
url https://doi.org/10.1038/s41467-021-25638-9
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