Excess charge-carrier induced instability of hybrid perovskites

Optoelectronic devices based on organic–inorganic halide perovskites show promising performance, but their poor stability impedes the commercialization. Here Lin et al. show that excess free charges are detrimental and efficient charge-carrier extraction is necessary for improved device stability.

Bibliographic Details
Main Authors: Yuze Lin, Bo Chen, Yanjun Fang, Jingjing Zhao, Chunxiong Bao, Zhenhua Yu, Yehao Deng, Peter N. Rudd, Yanfa Yan, Yongbo Yuan, Jinsong Huang
Format: Article
Language:English
Published: Nature Publishing Group 2018-11-01
Series:Nature Communications
Online Access:https://doi.org/10.1038/s41467-018-07438-w
id doaj-1c2d798f7a0d4733ae975fd2a712b8d4
record_format Article
spelling doaj-1c2d798f7a0d4733ae975fd2a712b8d42021-05-11T10:24:39ZengNature Publishing GroupNature Communications2041-17232018-11-01911910.1038/s41467-018-07438-wExcess charge-carrier induced instability of hybrid perovskitesYuze Lin0Bo Chen1Yanjun Fang2Jingjing Zhao3Chunxiong Bao4Zhenhua Yu5Yehao Deng6Peter N. Rudd7Yanfa Yan8Yongbo Yuan9Jinsong Huang10Department of Applied Physical Sciences, University of North CarolinaDepartment of Mechanical and Materials Engineering, and Nebraska Center for Materials and Nanoscience, University of Nebraska-LincolnDepartment of Mechanical and Materials Engineering, and Nebraska Center for Materials and Nanoscience, University of Nebraska-LincolnDepartment of Applied Physical Sciences, University of North CarolinaDepartment of Mechanical and Materials Engineering, and Nebraska Center for Materials and Nanoscience, University of Nebraska-LincolnDepartment of Applied Physical Sciences, University of North CarolinaDepartment of Applied Physical Sciences, University of North CarolinaDepartment of Applied Physical Sciences, University of North CarolinaDepartment of Physics and Astronomy, and Wright Center for Photovoltaics Innovation and Commercialization, The University of ToledoHunan Key Laboratory of Super Microstructure and Ultrafast Process, School of Physics and Electronics, Central South UniversityDepartment of Applied Physical Sciences, University of North CarolinaOptoelectronic devices based on organic–inorganic halide perovskites show promising performance, but their poor stability impedes the commercialization. Here Lin et al. show that excess free charges are detrimental and efficient charge-carrier extraction is necessary for improved device stability.https://doi.org/10.1038/s41467-018-07438-w
collection DOAJ
language English
format Article
sources DOAJ
author Yuze Lin
Bo Chen
Yanjun Fang
Jingjing Zhao
Chunxiong Bao
Zhenhua Yu
Yehao Deng
Peter N. Rudd
Yanfa Yan
Yongbo Yuan
Jinsong Huang
spellingShingle Yuze Lin
Bo Chen
Yanjun Fang
Jingjing Zhao
Chunxiong Bao
Zhenhua Yu
Yehao Deng
Peter N. Rudd
Yanfa Yan
Yongbo Yuan
Jinsong Huang
Excess charge-carrier induced instability of hybrid perovskites
Nature Communications
author_facet Yuze Lin
Bo Chen
Yanjun Fang
Jingjing Zhao
Chunxiong Bao
Zhenhua Yu
Yehao Deng
Peter N. Rudd
Yanfa Yan
Yongbo Yuan
Jinsong Huang
author_sort Yuze Lin
title Excess charge-carrier induced instability of hybrid perovskites
title_short Excess charge-carrier induced instability of hybrid perovskites
title_full Excess charge-carrier induced instability of hybrid perovskites
title_fullStr Excess charge-carrier induced instability of hybrid perovskites
title_full_unstemmed Excess charge-carrier induced instability of hybrid perovskites
title_sort excess charge-carrier induced instability of hybrid perovskites
publisher Nature Publishing Group
series Nature Communications
issn 2041-1723
publishDate 2018-11-01
description Optoelectronic devices based on organic–inorganic halide perovskites show promising performance, but their poor stability impedes the commercialization. Here Lin et al. show that excess free charges are detrimental and efficient charge-carrier extraction is necessary for improved device stability.
url https://doi.org/10.1038/s41467-018-07438-w
work_keys_str_mv AT yuzelin excesschargecarrierinducedinstabilityofhybridperovskites
AT bochen excesschargecarrierinducedinstabilityofhybridperovskites
AT yanjunfang excesschargecarrierinducedinstabilityofhybridperovskites
AT jingjingzhao excesschargecarrierinducedinstabilityofhybridperovskites
AT chunxiongbao excesschargecarrierinducedinstabilityofhybridperovskites
AT zhenhuayu excesschargecarrierinducedinstabilityofhybridperovskites
AT yehaodeng excesschargecarrierinducedinstabilityofhybridperovskites
AT peternrudd excesschargecarrierinducedinstabilityofhybridperovskites
AT yanfayan excesschargecarrierinducedinstabilityofhybridperovskites
AT yongboyuan excesschargecarrierinducedinstabilityofhybridperovskites
AT jinsonghuang excesschargecarrierinducedinstabilityofhybridperovskites
_version_ 1721448249401802752