Dopant-tuned stabilization of intermediates promotes electrosynthesis of valuable C3 products
The electro-oxidative synthesis of valued chemicals offers to enhance the overall efficiency and economic viability of renewable electrosynthesis systems. Here, the authors use dopant-tuned catalysts to promote the electrosynthesis of dimethyl carbonate from CO and methanol via oxidative carbonylati...
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Online Access: | https://doi.org/10.1038/s41467-019-12788-0 |
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doaj-35211011e6c74184a1edf77d819c08e02021-05-11T12:40:25ZengNature Publishing GroupNature Communications2041-17232019-10-011011710.1038/s41467-019-12788-0Dopant-tuned stabilization of intermediates promotes electrosynthesis of valuable C3 productsTao-Tao Zhuang0Dae-Hyun Nam1Ziyun Wang2Hui-Hui Li3Christine M. Gabardo4Yi Li5Zhi-Qin Liang6Jun Li7Xiao-Jing Liu8Bin Chen9Wan Ru Leow10Rui Wu11Xue Wang12Fengwang Li13Yanwei Lum14Joshua Wicks15Colin P. O’Brien16Tao Peng17Alexander H. Ip18Tsun-Kong Sham19Shu-Hong Yu20David Sinton21Edward H. Sargent22Department of Electrical and Computer Engineering, University of TorontoDepartment of Electrical and Computer Engineering, University of TorontoDepartment of Electrical and Computer Engineering, University of TorontoDepartment of Electrical and Computer Engineering, University of TorontoDepartment of Mechanical and Industrial Engineering, University of TorontoDivision of Nanomaterials & Chemistry, Hefei National Laboratory for Physical Sciences at Microscale, Collaborative Innovation Center of Suzhou Nano Science and Technology, CAS Center for Excellence in Nanoscience, Department of Chemistry, University of Science and Technology of ChinaDepartment of Electrical and Computer Engineering, University of TorontoDepartment of Electrical and Computer Engineering, University of TorontoDivision of Nanomaterials & Chemistry, Hefei National Laboratory for Physical Sciences at Microscale, Collaborative Innovation Center of Suzhou Nano Science and Technology, CAS Center for Excellence in Nanoscience, Department of Chemistry, University of Science and Technology of ChinaDepartment of Electrical and Computer Engineering, University of TorontoDepartment of Electrical and Computer Engineering, University of TorontoDivision of Nanomaterials & Chemistry, Hefei National Laboratory for Physical Sciences at Microscale, Collaborative Innovation Center of Suzhou Nano Science and Technology, CAS Center for Excellence in Nanoscience, Department of Chemistry, University of Science and Technology of ChinaDepartment of Electrical and Computer Engineering, University of TorontoDepartment of Electrical and Computer Engineering, University of TorontoDepartment of Electrical and Computer Engineering, University of TorontoDepartment of Electrical and Computer Engineering, University of TorontoDepartment of Mechanical and Industrial Engineering, University of TorontoDepartment of Electrical and Computer Engineering, University of TorontoDepartment of Electrical and Computer Engineering, University of TorontoDepartment of Chemistry, University of Western OntarioDivision of Nanomaterials & Chemistry, Hefei National Laboratory for Physical Sciences at Microscale, Collaborative Innovation Center of Suzhou Nano Science and Technology, CAS Center for Excellence in Nanoscience, Department of Chemistry, University of Science and Technology of ChinaDepartment of Mechanical and Industrial Engineering, University of TorontoDepartment of Electrical and Computer Engineering, University of TorontoThe electro-oxidative synthesis of valued chemicals offers to enhance the overall efficiency and economic viability of renewable electrosynthesis systems. Here, the authors use dopant-tuned catalysts to promote the electrosynthesis of dimethyl carbonate from CO and methanol via oxidative carbonylation.https://doi.org/10.1038/s41467-019-12788-0 |
collection |
DOAJ |
language |
English |
format |
Article |
sources |
DOAJ |
author |
Tao-Tao Zhuang Dae-Hyun Nam Ziyun Wang Hui-Hui Li Christine M. Gabardo Yi Li Zhi-Qin Liang Jun Li Xiao-Jing Liu Bin Chen Wan Ru Leow Rui Wu Xue Wang Fengwang Li Yanwei Lum Joshua Wicks Colin P. O’Brien Tao Peng Alexander H. Ip Tsun-Kong Sham Shu-Hong Yu David Sinton Edward H. Sargent |
spellingShingle |
Tao-Tao Zhuang Dae-Hyun Nam Ziyun Wang Hui-Hui Li Christine M. Gabardo Yi Li Zhi-Qin Liang Jun Li Xiao-Jing Liu Bin Chen Wan Ru Leow Rui Wu Xue Wang Fengwang Li Yanwei Lum Joshua Wicks Colin P. O’Brien Tao Peng Alexander H. Ip Tsun-Kong Sham Shu-Hong Yu David Sinton Edward H. Sargent Dopant-tuned stabilization of intermediates promotes electrosynthesis of valuable C3 products Nature Communications |
author_facet |
Tao-Tao Zhuang Dae-Hyun Nam Ziyun Wang Hui-Hui Li Christine M. Gabardo Yi Li Zhi-Qin Liang Jun Li Xiao-Jing Liu Bin Chen Wan Ru Leow Rui Wu Xue Wang Fengwang Li Yanwei Lum Joshua Wicks Colin P. O’Brien Tao Peng Alexander H. Ip Tsun-Kong Sham Shu-Hong Yu David Sinton Edward H. Sargent |
author_sort |
Tao-Tao Zhuang |
title |
Dopant-tuned stabilization of intermediates promotes electrosynthesis of valuable C3 products |
title_short |
Dopant-tuned stabilization of intermediates promotes electrosynthesis of valuable C3 products |
title_full |
Dopant-tuned stabilization of intermediates promotes electrosynthesis of valuable C3 products |
title_fullStr |
Dopant-tuned stabilization of intermediates promotes electrosynthesis of valuable C3 products |
title_full_unstemmed |
Dopant-tuned stabilization of intermediates promotes electrosynthesis of valuable C3 products |
title_sort |
dopant-tuned stabilization of intermediates promotes electrosynthesis of valuable c3 products |
publisher |
Nature Publishing Group |
series |
Nature Communications |
issn |
2041-1723 |
publishDate |
2019-10-01 |
description |
The electro-oxidative synthesis of valued chemicals offers to enhance the overall efficiency and economic viability of renewable electrosynthesis systems. Here, the authors use dopant-tuned catalysts to promote the electrosynthesis of dimethyl carbonate from CO and methanol via oxidative carbonylation. |
url |
https://doi.org/10.1038/s41467-019-12788-0 |
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