Understanding carbon dioxide activation and carbon–carbon coupling over nickel

Carbon dioxide is a desired feedstock for platform molecules, such as carbon monoxide and higher hydrocarbons, but needs improved catalysts. Here, the authors use a combined theoretical and experimental approach to tune the activity and selectivity of CO2 conversion over nickel towards desired produ...

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Main Authors: Charlotte Vogt, Matteo Monai, Ellen B. Sterk, Jonas Palle, Angela E. M. Melcherts, Bart Zijlstra, Esther Groeneveld, Peter H. Berben, Jelle M. Boereboom, Emiel J. M. Hensen, Florian Meirer, Ivo A. W. Filot, Bert M. Weckhuysen
Format: Article
Language:English
Published: Nature Publishing Group 2019-11-01
Series:Nature Communications
Online Access:https://doi.org/10.1038/s41467-019-12858-3
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spelling doaj-450d9c4d27154d0bb0e8e3fc2a1c8e8a2021-05-11T11:38:58ZengNature Publishing GroupNature Communications2041-17232019-11-0110111010.1038/s41467-019-12858-3Understanding carbon dioxide activation and carbon–carbon coupling over nickelCharlotte Vogt0Matteo Monai1Ellen B. Sterk2Jonas Palle3Angela E. M. Melcherts4Bart Zijlstra5Esther Groeneveld6Peter H. Berben7Jelle M. Boereboom8Emiel J. M. Hensen9Florian Meirer10Ivo A. W. Filot11Bert M. Weckhuysen12Inorganic Chemistry and Catalysis group, Debye Institute for Nanomaterials Science, Utrecht UniversityInorganic Chemistry and Catalysis group, Debye Institute for Nanomaterials Science, Utrecht UniversityInorganic Chemistry and Catalysis group, Debye Institute for Nanomaterials Science, Utrecht UniversityInorganic Chemistry and Catalysis group, Debye Institute for Nanomaterials Science, Utrecht UniversityInorganic Chemistry and Catalysis group, Debye Institute for Nanomaterials Science, Utrecht UniversitySchuit Institute of Catalysis, Department of Chemical Engineering and Chemistry, Eindhoven University of TechnologyBASF Nederland B.V.BASF Nederland B.V.Inorganic Chemistry and Catalysis group, Debye Institute for Nanomaterials Science, Utrecht UniversitySchuit Institute of Catalysis, Department of Chemical Engineering and Chemistry, Eindhoven University of TechnologyInorganic Chemistry and Catalysis group, Debye Institute for Nanomaterials Science, Utrecht UniversitySchuit Institute of Catalysis, Department of Chemical Engineering and Chemistry, Eindhoven University of TechnologyInorganic Chemistry and Catalysis group, Debye Institute for Nanomaterials Science, Utrecht UniversityCarbon dioxide is a desired feedstock for platform molecules, such as carbon monoxide and higher hydrocarbons, but needs improved catalysts. Here, the authors use a combined theoretical and experimental approach to tune the activity and selectivity of CO2 conversion over nickel towards desired products.https://doi.org/10.1038/s41467-019-12858-3
collection DOAJ
language English
format Article
sources DOAJ
author Charlotte Vogt
Matteo Monai
Ellen B. Sterk
Jonas Palle
Angela E. M. Melcherts
Bart Zijlstra
Esther Groeneveld
Peter H. Berben
Jelle M. Boereboom
Emiel J. M. Hensen
Florian Meirer
Ivo A. W. Filot
Bert M. Weckhuysen
spellingShingle Charlotte Vogt
Matteo Monai
Ellen B. Sterk
Jonas Palle
Angela E. M. Melcherts
Bart Zijlstra
Esther Groeneveld
Peter H. Berben
Jelle M. Boereboom
Emiel J. M. Hensen
Florian Meirer
Ivo A. W. Filot
Bert M. Weckhuysen
Understanding carbon dioxide activation and carbon–carbon coupling over nickel
Nature Communications
author_facet Charlotte Vogt
Matteo Monai
Ellen B. Sterk
Jonas Palle
Angela E. M. Melcherts
Bart Zijlstra
Esther Groeneveld
Peter H. Berben
Jelle M. Boereboom
Emiel J. M. Hensen
Florian Meirer
Ivo A. W. Filot
Bert M. Weckhuysen
author_sort Charlotte Vogt
title Understanding carbon dioxide activation and carbon–carbon coupling over nickel
title_short Understanding carbon dioxide activation and carbon–carbon coupling over nickel
title_full Understanding carbon dioxide activation and carbon–carbon coupling over nickel
title_fullStr Understanding carbon dioxide activation and carbon–carbon coupling over nickel
title_full_unstemmed Understanding carbon dioxide activation and carbon–carbon coupling over nickel
title_sort understanding carbon dioxide activation and carbon–carbon coupling over nickel
publisher Nature Publishing Group
series Nature Communications
issn 2041-1723
publishDate 2019-11-01
description Carbon dioxide is a desired feedstock for platform molecules, such as carbon monoxide and higher hydrocarbons, but needs improved catalysts. Here, the authors use a combined theoretical and experimental approach to tune the activity and selectivity of CO2 conversion over nickel towards desired products.
url https://doi.org/10.1038/s41467-019-12858-3
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