Optical spin-state polarization in a binuclear europium complex towards molecule-based coherent light-spin interfaces

Rare-earth ion (REI)-doped systems are well suited for realising coherent light-spin interfaces, but demonstrations of spectral hole burning (SHB) in optical transitions of REI-based systems have been so far limited to REIs dispersed in matrices. Here, the authors report on transient SHB in a binucl...

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Main Authors: Kuppusamy Senthil Kumar, Diana Serrano, Aline M. Nonat, Benoît Heinrich, Lydia Karmazin, Loïc J. Charbonnière, Philippe Goldner, Mario Ruben
Format: Article
Language:English
Published: Nature Publishing Group 2021-04-01
Series:Nature Communications
Online Access:https://doi.org/10.1038/s41467-021-22383-x
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spelling doaj-5ea7e3d5ffc349818744fbb30f4ed6092021-04-18T11:12:49ZengNature Publishing GroupNature Communications2041-17232021-04-011211710.1038/s41467-021-22383-xOptical spin-state polarization in a binuclear europium complex towards molecule-based coherent light-spin interfacesKuppusamy Senthil Kumar0Diana Serrano1Aline M. Nonat2Benoît Heinrich3Lydia Karmazin4Loïc J. Charbonnière5Philippe Goldner6Mario Ruben7Institut de Physique et Chimie des Matériaux de Strasbourg (IPCMS), CNRS-Université de StrasbourgInstitut de Recherche de Chimie Paris (IRCP), Université PSL, Chimie ParisTech, CNRSEquipe de Synthèse pour l’Analyse, IPHC, UMR 7178, CNRS‐Université de Strasbourg, ECPMInstitut de Physique et Chimie des Matériaux de Strasbourg (IPCMS), CNRS-Université de StrasbourgService de Radiocristallographie, Fédération de Chimie Le Bel FR2010 CNRS-Université de StrasbourgEquipe de Synthèse pour l’Analyse, IPHC, UMR 7178, CNRS‐Université de Strasbourg, ECPMInstitut de Recherche de Chimie Paris (IRCP), Université PSL, Chimie ParisTech, CNRSInstitute of Nanotechnology, Karlsruhe Institute of Technology (KIT)Rare-earth ion (REI)-doped systems are well suited for realising coherent light-spin interfaces, but demonstrations of spectral hole burning (SHB) in optical transitions of REI-based systems have been so far limited to REIs dispersed in matrices. Here, the authors report on transient SHB in a binuclear Eu(III) complex.https://doi.org/10.1038/s41467-021-22383-x
collection DOAJ
language English
format Article
sources DOAJ
author Kuppusamy Senthil Kumar
Diana Serrano
Aline M. Nonat
Benoît Heinrich
Lydia Karmazin
Loïc J. Charbonnière
Philippe Goldner
Mario Ruben
spellingShingle Kuppusamy Senthil Kumar
Diana Serrano
Aline M. Nonat
Benoît Heinrich
Lydia Karmazin
Loïc J. Charbonnière
Philippe Goldner
Mario Ruben
Optical spin-state polarization in a binuclear europium complex towards molecule-based coherent light-spin interfaces
Nature Communications
author_facet Kuppusamy Senthil Kumar
Diana Serrano
Aline M. Nonat
Benoît Heinrich
Lydia Karmazin
Loïc J. Charbonnière
Philippe Goldner
Mario Ruben
author_sort Kuppusamy Senthil Kumar
title Optical spin-state polarization in a binuclear europium complex towards molecule-based coherent light-spin interfaces
title_short Optical spin-state polarization in a binuclear europium complex towards molecule-based coherent light-spin interfaces
title_full Optical spin-state polarization in a binuclear europium complex towards molecule-based coherent light-spin interfaces
title_fullStr Optical spin-state polarization in a binuclear europium complex towards molecule-based coherent light-spin interfaces
title_full_unstemmed Optical spin-state polarization in a binuclear europium complex towards molecule-based coherent light-spin interfaces
title_sort optical spin-state polarization in a binuclear europium complex towards molecule-based coherent light-spin interfaces
publisher Nature Publishing Group
series Nature Communications
issn 2041-1723
publishDate 2021-04-01
description Rare-earth ion (REI)-doped systems are well suited for realising coherent light-spin interfaces, but demonstrations of spectral hole burning (SHB) in optical transitions of REI-based systems have been so far limited to REIs dispersed in matrices. Here, the authors report on transient SHB in a binuclear Eu(III) complex.
url https://doi.org/10.1038/s41467-021-22383-x
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