Fabrication and temperature-dependent electrical characterization of a C-shape nanowire patterned by a DNA origami

Abstract We introduce a method based on directed molecular self-assembly to manufacture and electrically characterise C-shape gold nanowires which clearly deviate from typical linear shape due to the design of the template guiding the assembly. To this end, gold nanoparticles are arranged in the des...

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Main Authors: Türkan Bayrak, Amanda Martinez-Reyes, David Daniel Ruiz Arce, Jeffrey Kelling, Enrique C Samano, Artur Erbe
Format: Article
Language:English
Published: Nature Publishing Group 2021-01-01
Series:Scientific Reports
Online Access:https://doi.org/10.1038/s41598-021-81178-8
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spelling doaj-60282b5b722442afad1dd928172d27a52021-01-24T12:29:53ZengNature Publishing GroupScientific Reports2045-23222021-01-011111910.1038/s41598-021-81178-8Fabrication and temperature-dependent electrical characterization of a C-shape nanowire patterned by a DNA origamiTürkan Bayrak0Amanda Martinez-Reyes1David Daniel Ruiz Arce2Jeffrey Kelling3Enrique C Samano4Artur Erbe5Institute of Ion Beam Physics and Materials Research, Helmholtz-Zentrum Dresden-RossendorfCentro de Nanociencias y Nanotecnologia, Universidad Nacional Autonoma de MexicoCentro de Nanociencias y Nanotecnologia, Universidad Nacional Autonoma de MexicoDepartment of Information Services and Computing, Helmholtz-Zentrum Dresden-RossendorfCentro de Nanociencias y Nanotecnologia, Universidad Nacional Autonoma de MexicoInstitute of Ion Beam Physics and Materials Research, Helmholtz-Zentrum Dresden-RossendorfAbstract We introduce a method based on directed molecular self-assembly to manufacture and electrically characterise C-shape gold nanowires which clearly deviate from typical linear shape due to the design of the template guiding the assembly. To this end, gold nanoparticles are arranged in the desired shape on a DNA-origami template and enhanced to form a continuous wire through electroless deposition. C-shape nanowires with a size below 150nm on a $${\hbox {SiO}_2}/\hbox {Si}$$ SiO 2 / Si substrate are contacted with gold electrodes by means of electron beam lithography. Charge transport measurements of the nanowires show hopping, thermionic and tunneling transports at different temperatures in the 4.2K to 293K range. The different transport mechanisms indicate that the C-shape nanowires consist of metallic segments which are weakly coupled along the wires.https://doi.org/10.1038/s41598-021-81178-8
collection DOAJ
language English
format Article
sources DOAJ
author Türkan Bayrak
Amanda Martinez-Reyes
David Daniel Ruiz Arce
Jeffrey Kelling
Enrique C Samano
Artur Erbe
spellingShingle Türkan Bayrak
Amanda Martinez-Reyes
David Daniel Ruiz Arce
Jeffrey Kelling
Enrique C Samano
Artur Erbe
Fabrication and temperature-dependent electrical characterization of a C-shape nanowire patterned by a DNA origami
Scientific Reports
author_facet Türkan Bayrak
Amanda Martinez-Reyes
David Daniel Ruiz Arce
Jeffrey Kelling
Enrique C Samano
Artur Erbe
author_sort Türkan Bayrak
title Fabrication and temperature-dependent electrical characterization of a C-shape nanowire patterned by a DNA origami
title_short Fabrication and temperature-dependent electrical characterization of a C-shape nanowire patterned by a DNA origami
title_full Fabrication and temperature-dependent electrical characterization of a C-shape nanowire patterned by a DNA origami
title_fullStr Fabrication and temperature-dependent electrical characterization of a C-shape nanowire patterned by a DNA origami
title_full_unstemmed Fabrication and temperature-dependent electrical characterization of a C-shape nanowire patterned by a DNA origami
title_sort fabrication and temperature-dependent electrical characterization of a c-shape nanowire patterned by a dna origami
publisher Nature Publishing Group
series Scientific Reports
issn 2045-2322
publishDate 2021-01-01
description Abstract We introduce a method based on directed molecular self-assembly to manufacture and electrically characterise C-shape gold nanowires which clearly deviate from typical linear shape due to the design of the template guiding the assembly. To this end, gold nanoparticles are arranged in the desired shape on a DNA-origami template and enhanced to form a continuous wire through electroless deposition. C-shape nanowires with a size below 150nm on a $${\hbox {SiO}_2}/\hbox {Si}$$ SiO 2 / Si substrate are contacted with gold electrodes by means of electron beam lithography. Charge transport measurements of the nanowires show hopping, thermionic and tunneling transports at different temperatures in the 4.2K to 293K range. The different transport mechanisms indicate that the C-shape nanowires consist of metallic segments which are weakly coupled along the wires.
url https://doi.org/10.1038/s41598-021-81178-8
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