Identifying the nature of the active sites in methanol synthesis over Cu/ZnO/Al2O3 catalysts

Methanol synthesis has a high potential for global CO2 reduction. Here, the authors identify the oxidation state of the zinc sites on the metallic copper particles as partially positive for an industrial Cu/ZnO/Al2O3 catalyst under high-pressure reaction conditions.

Bibliographic Details
Main Authors: Daniel Laudenschleger, Holger Ruland, Martin Muhler
Format: Article
Language:English
Published: Nature Publishing Group 2020-08-01
Series:Nature Communications
Online Access:https://doi.org/10.1038/s41467-020-17631-5
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spelling doaj-6d3b4c2ea8834533bed11128ae0c49fa2021-08-08T11:39:08ZengNature Publishing GroupNature Communications2041-17232020-08-0111111010.1038/s41467-020-17631-5Identifying the nature of the active sites in methanol synthesis over Cu/ZnO/Al2O3 catalystsDaniel Laudenschleger0Holger Ruland1Martin Muhler2Laboratory of Industrial Chemistry, Ruhr University Bochum, Universitätsstraße 150Max Planck Institute for Chemical Energy ConversionLaboratory of Industrial Chemistry, Ruhr University Bochum, Universitätsstraße 150Methanol synthesis has a high potential for global CO2 reduction. Here, the authors identify the oxidation state of the zinc sites on the metallic copper particles as partially positive for an industrial Cu/ZnO/Al2O3 catalyst under high-pressure reaction conditions.https://doi.org/10.1038/s41467-020-17631-5
collection DOAJ
language English
format Article
sources DOAJ
author Daniel Laudenschleger
Holger Ruland
Martin Muhler
spellingShingle Daniel Laudenschleger
Holger Ruland
Martin Muhler
Identifying the nature of the active sites in methanol synthesis over Cu/ZnO/Al2O3 catalysts
Nature Communications
author_facet Daniel Laudenschleger
Holger Ruland
Martin Muhler
author_sort Daniel Laudenschleger
title Identifying the nature of the active sites in methanol synthesis over Cu/ZnO/Al2O3 catalysts
title_short Identifying the nature of the active sites in methanol synthesis over Cu/ZnO/Al2O3 catalysts
title_full Identifying the nature of the active sites in methanol synthesis over Cu/ZnO/Al2O3 catalysts
title_fullStr Identifying the nature of the active sites in methanol synthesis over Cu/ZnO/Al2O3 catalysts
title_full_unstemmed Identifying the nature of the active sites in methanol synthesis over Cu/ZnO/Al2O3 catalysts
title_sort identifying the nature of the active sites in methanol synthesis over cu/zno/al2o3 catalysts
publisher Nature Publishing Group
series Nature Communications
issn 2041-1723
publishDate 2020-08-01
description Methanol synthesis has a high potential for global CO2 reduction. Here, the authors identify the oxidation state of the zinc sites on the metallic copper particles as partially positive for an industrial Cu/ZnO/Al2O3 catalyst under high-pressure reaction conditions.
url https://doi.org/10.1038/s41467-020-17631-5
work_keys_str_mv AT daniellaudenschleger identifyingthenatureoftheactivesitesinmethanolsynthesisovercuznoal2o3catalysts
AT holgerruland identifyingthenatureoftheactivesitesinmethanolsynthesisovercuznoal2o3catalysts
AT martinmuhler identifyingthenatureoftheactivesitesinmethanolsynthesisovercuznoal2o3catalysts
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