The description and validation of the computationally Efficient CH<sub>4</sub>–CO–OH (ECCOHv1.01) chemistry module for 3-D model applications

We present the Efficient CH<sub>4</sub>–CO–OH (ECCOH) chemistry module that allows for the simulation of the methane, carbon monoxide, and hydroxyl radical (CH<sub>4</sub>–CO–OH) system, within a chemistry climate model, carbon cycle model, or Earth system model. The computat...

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Bibliographic Details
Main Authors: Y. F. Elshorbany, B. N. Duncan, S. A. Strode, J. S. Wang, J. Kouatchou
Format: Article
Language:English
Published: Copernicus Publications 2016-02-01
Series:Geoscientific Model Development
Online Access:http://www.geosci-model-dev.net/9/799/2016/gmd-9-799-2016.pdf
Description
Summary:We present the Efficient CH<sub>4</sub>–CO–OH (ECCOH) chemistry module that allows for the simulation of the methane, carbon monoxide, and hydroxyl radical (CH<sub>4</sub>–CO–OH) system, within a chemistry climate model, carbon cycle model, or Earth system model. The computational efficiency of the module allows many multi-decadal sensitivity simulations of the CH<sub>4</sub>–CO–OH system, which primarily determines the global atmospheric oxidizing capacity. This capability is important for capturing the nonlinear feedbacks of the CH<sub>4</sub>–CO–OH system and understanding the perturbations to methane, CO, and OH, and the concomitant impacts on climate. We implemented the ECCOH chemistry module in the NASA GEOS-5 atmospheric global circulation model (AGCM), performed multiple sensitivity simulations of the CH<sub>4</sub>–CO–OH system over 2 decades, and evaluated the model output with surface and satellite data sets of methane and CO. The favorable comparison of output from the ECCOH chemistry module (as configured in the GEOS-5 AGCM) with observations demonstrates the fidelity of the module for use in scientific research.
ISSN:1991-959X
1991-9603