Enhanced Visible-Light Photocatalysis of Nanocomposites of Copper Oxide and Single-Walled Carbon Nanotubes for the Degradation of Methylene Blue

We report enhanced catalytic action of a series of copper(II)-oxide-single-walled carbon nanotube (CuO-SWCNT) composite photocatalysts (abbreviated as CuO-SWCNT-0.5, CuO-SWCNT-2, and CuO-SWCNT-5, where 0.5, 2, and 5 represent the calcination time in hours) synthesized via recrystallization followed...

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Main Authors: Kamal Prasad Sapkota, Insup Lee, Md. Abu Hanif, Md. Akherul Islam, Jeasmin Akter, Jae Ryang Hahn
Format: Article
Language:English
Published: MDPI AG 2020-03-01
Series:Catalysts
Subjects:
Online Access:https://www.mdpi.com/2073-4344/10/3/297
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spelling doaj-82080aac2edf4aafae0d9da15d2aaec52020-11-25T02:28:13ZengMDPI AGCatalysts2073-43442020-03-0110329710.3390/catal10030297catal10030297Enhanced Visible-Light Photocatalysis of Nanocomposites of Copper Oxide and Single-Walled Carbon Nanotubes for the Degradation of Methylene BlueKamal Prasad Sapkota0Insup Lee1Md. Abu Hanif2Md. Akherul Islam3Jeasmin Akter4Jae Ryang Hahn5Department of Chemistry and Bioactive Material Sciences, Research Institute of Physics and Chemistry, Jeonbuk National University, Jeonju 54896, KoreaDepartment of Chemistry and Bioactive Material Sciences, Research Institute of Physics and Chemistry, Jeonbuk National University, Jeonju 54896, KoreaDepartment of Chemistry and Bioactive Material Sciences, Research Institute of Physics and Chemistry, Jeonbuk National University, Jeonju 54896, KoreaDepartment of Chemistry and Bioactive Material Sciences, Research Institute of Physics and Chemistry, Jeonbuk National University, Jeonju 54896, KoreaDepartment of Chemistry and Bioactive Material Sciences, Research Institute of Physics and Chemistry, Jeonbuk National University, Jeonju 54896, KoreaDepartment of Chemistry and Bioactive Material Sciences, Research Institute of Physics and Chemistry, Jeonbuk National University, Jeonju 54896, KoreaWe report enhanced catalytic action of a series of copper(II)-oxide-single-walled carbon nanotube (CuO-SWCNT) composite photocatalysts (abbreviated as CuO-SWCNT-0.5, CuO-SWCNT-2, and CuO-SWCNT-5, where 0.5, 2, and 5 represent the calcination time in hours) synthesized via recrystallization followed by calcination. The photocatalytic performance of the fabricated nanocomposites was examined by evaluating the degradation of methylene blue (MB) under irradiation with visible light. All of the as-fabricated nanocomposites were effective photocatalysts for the photodegradation of a MB solution; however, the CuO-SWCNT-5 displayed the best photocatalytic ability among the investigated catalysts, achieving 97.33% degradation of MB in 2 h under visible-light irradiation. The photocatalytic action of the nanocomposites was remarkably higher than that of pristine CuO nanocrystals fabricated using the same route. The recyclability of the photocatalyst was also investigated; the CuO-SWCNT-5 catalyst could be reused for three cycles without substantial degradation of its catalytic performance or morphology.https://www.mdpi.com/2073-4344/10/3/297cuo-swcnt nanocompositesrecrystallizationmethylene bluephotocatalystvisible light photocatalysisdecomposition
collection DOAJ
language English
format Article
sources DOAJ
author Kamal Prasad Sapkota
Insup Lee
Md. Abu Hanif
Md. Akherul Islam
Jeasmin Akter
Jae Ryang Hahn
spellingShingle Kamal Prasad Sapkota
Insup Lee
Md. Abu Hanif
Md. Akherul Islam
Jeasmin Akter
Jae Ryang Hahn
Enhanced Visible-Light Photocatalysis of Nanocomposites of Copper Oxide and Single-Walled Carbon Nanotubes for the Degradation of Methylene Blue
Catalysts
cuo-swcnt nanocomposites
recrystallization
methylene blue
photocatalyst
visible light photocatalysis
decomposition
author_facet Kamal Prasad Sapkota
Insup Lee
Md. Abu Hanif
Md. Akherul Islam
Jeasmin Akter
Jae Ryang Hahn
author_sort Kamal Prasad Sapkota
title Enhanced Visible-Light Photocatalysis of Nanocomposites of Copper Oxide and Single-Walled Carbon Nanotubes for the Degradation of Methylene Blue
title_short Enhanced Visible-Light Photocatalysis of Nanocomposites of Copper Oxide and Single-Walled Carbon Nanotubes for the Degradation of Methylene Blue
title_full Enhanced Visible-Light Photocatalysis of Nanocomposites of Copper Oxide and Single-Walled Carbon Nanotubes for the Degradation of Methylene Blue
title_fullStr Enhanced Visible-Light Photocatalysis of Nanocomposites of Copper Oxide and Single-Walled Carbon Nanotubes for the Degradation of Methylene Blue
title_full_unstemmed Enhanced Visible-Light Photocatalysis of Nanocomposites of Copper Oxide and Single-Walled Carbon Nanotubes for the Degradation of Methylene Blue
title_sort enhanced visible-light photocatalysis of nanocomposites of copper oxide and single-walled carbon nanotubes for the degradation of methylene blue
publisher MDPI AG
series Catalysts
issn 2073-4344
publishDate 2020-03-01
description We report enhanced catalytic action of a series of copper(II)-oxide-single-walled carbon nanotube (CuO-SWCNT) composite photocatalysts (abbreviated as CuO-SWCNT-0.5, CuO-SWCNT-2, and CuO-SWCNT-5, where 0.5, 2, and 5 represent the calcination time in hours) synthesized via recrystallization followed by calcination. The photocatalytic performance of the fabricated nanocomposites was examined by evaluating the degradation of methylene blue (MB) under irradiation with visible light. All of the as-fabricated nanocomposites were effective photocatalysts for the photodegradation of a MB solution; however, the CuO-SWCNT-5 displayed the best photocatalytic ability among the investigated catalysts, achieving 97.33% degradation of MB in 2 h under visible-light irradiation. The photocatalytic action of the nanocomposites was remarkably higher than that of pristine CuO nanocrystals fabricated using the same route. The recyclability of the photocatalyst was also investigated; the CuO-SWCNT-5 catalyst could be reused for three cycles without substantial degradation of its catalytic performance or morphology.
topic cuo-swcnt nanocomposites
recrystallization
methylene blue
photocatalyst
visible light photocatalysis
decomposition
url https://www.mdpi.com/2073-4344/10/3/297
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AT insuplee enhancedvisiblelightphotocatalysisofnanocompositesofcopperoxideandsinglewalledcarbonnanotubesforthedegradationofmethyleneblue
AT mdabuhanif enhancedvisiblelightphotocatalysisofnanocompositesofcopperoxideandsinglewalledcarbonnanotubesforthedegradationofmethyleneblue
AT mdakherulislam enhancedvisiblelightphotocatalysisofnanocompositesofcopperoxideandsinglewalledcarbonnanotubesforthedegradationofmethyleneblue
AT jeasminakter enhancedvisiblelightphotocatalysisofnanocompositesofcopperoxideandsinglewalledcarbonnanotubesforthedegradationofmethyleneblue
AT jaeryanghahn enhancedvisiblelightphotocatalysisofnanocompositesofcopperoxideandsinglewalledcarbonnanotubesforthedegradationofmethyleneblue
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