Stimulated Raman Scattering in Alkali-Earth Tungstate and Molybdate Crystals at Both Stretching and Bending Raman Modes under Synchronous Picosecond Pumping with Multiple Pulse Shortening Down to 1 ps
Comparative investigation of characteristics of spontaneous and stimulated Raman scattering (SRS) in different alkali-earth tungstate and molybdate crystals at both high and low frequency anionic group vibrations is presented. It has been found that, among these crystals, the SrMoO<sub>4</s...
Main Authors: | , , , , , , , , , |
---|---|
Format: | Article |
Language: | English |
Published: |
MDPI AG
2019-03-01
|
Series: | Crystals |
Subjects: | |
Online Access: | https://www.mdpi.com/2073-4352/9/3/167 |
id |
doaj-8be554d8da8846bc9b964d4e86552f7e |
---|---|
record_format |
Article |
spelling |
doaj-8be554d8da8846bc9b964d4e86552f7e2020-11-24T22:11:29ZengMDPI AGCrystals2073-43522019-03-019316710.3390/cryst9030167cryst9030167Stimulated Raman Scattering in Alkali-Earth Tungstate and Molybdate Crystals at Both Stretching and Bending Raman Modes under Synchronous Picosecond Pumping with Multiple Pulse Shortening Down to 1 psMilan Frank0Sergei N. Smetanin1Michal Jelínek2David Vyhlídal3Vladislav E. Shukshin4Lyudmila I. Ivleva5Elizaveta E. Dunaeva6Irina S. Voronina7Petr G. Zverev8Václav Kubeček9Faculty of Nuclear Sciences and Physical Engineering, Czech Technical University, Břehová 7, 11519 Prague 1, Czech RepublicFaculty of Nuclear Sciences and Physical Engineering, Czech Technical University, Břehová 7, 11519 Prague 1, Czech RepublicFaculty of Nuclear Sciences and Physical Engineering, Czech Technical University, Břehová 7, 11519 Prague 1, Czech RepublicFaculty of Nuclear Sciences and Physical Engineering, Czech Technical University, Břehová 7, 11519 Prague 1, Czech RepublicProkhorov General Physics Institute of the Russian Academy of Sciences, Vavilova 38, 119991 Moscow, RussianProkhorov General Physics Institute of the Russian Academy of Sciences, Vavilova 38, 119991 Moscow, RussianProkhorov General Physics Institute of the Russian Academy of Sciences, Vavilova 38, 119991 Moscow, RussianProkhorov General Physics Institute of the Russian Academy of Sciences, Vavilova 38, 119991 Moscow, RussianProkhorov General Physics Institute of the Russian Academy of Sciences, Vavilova 38, 119991 Moscow, RussianFaculty of Nuclear Sciences and Physical Engineering, Czech Technical University, Břehová 7, 11519 Prague 1, Czech RepublicComparative investigation of characteristics of spontaneous and stimulated Raman scattering (SRS) in different alkali-earth tungstate and molybdate crystals at both high and low frequency anionic group vibrations is presented. It has been found that, among these crystals, the SrMoO<sub>4</sub> and SrWO<sub>4</sub> crystals are the most perspective for SRS generation on both stretching and bending modes of internal anionic group vibrations with the strongest SRS pulse shortening under synchronous laser pumping because of not only highly intense stretching mode Raman line for efficient primary extra cavity long-shifted SRS conversion but also the widest bending mode Raman line for the strongest SRS pulse shortening down to the inverse width of the widest Raman line (~1 ps) at secondary intracavity short-shifted SRS conversion. The strongest 26-fold pump pulse shortening down to 1.4 ps at the Stokes component with the combined Raman shift in the synchronously pumped extra cavity SrMoO<sub>4</sub> and SrWO<sub>4</sub> Raman lasers has been demonstrated. It was found that synchronously pumped cascade SRS with combined Raman shift is more efficient in the SrWO<sub>4</sub> crystal because the bending mode Raman line is more intense relative to the stretching mode Raman line than that in SrMoO<sub>4</sub>.https://www.mdpi.com/2073-4352/9/3/167alkali-earth tungstatemolybdate crystalsstretchingbending Raman modesstimulated Raman scattering |
collection |
DOAJ |
language |
English |
format |
Article |
sources |
DOAJ |
author |
Milan Frank Sergei N. Smetanin Michal Jelínek David Vyhlídal Vladislav E. Shukshin Lyudmila I. Ivleva Elizaveta E. Dunaeva Irina S. Voronina Petr G. Zverev Václav Kubeček |
spellingShingle |
Milan Frank Sergei N. Smetanin Michal Jelínek David Vyhlídal Vladislav E. Shukshin Lyudmila I. Ivleva Elizaveta E. Dunaeva Irina S. Voronina Petr G. Zverev Václav Kubeček Stimulated Raman Scattering in Alkali-Earth Tungstate and Molybdate Crystals at Both Stretching and Bending Raman Modes under Synchronous Picosecond Pumping with Multiple Pulse Shortening Down to 1 ps Crystals alkali-earth tungstate molybdate crystals stretching bending Raman modes stimulated Raman scattering |
author_facet |
Milan Frank Sergei N. Smetanin Michal Jelínek David Vyhlídal Vladislav E. Shukshin Lyudmila I. Ivleva Elizaveta E. Dunaeva Irina S. Voronina Petr G. Zverev Václav Kubeček |
author_sort |
Milan Frank |
title |
Stimulated Raman Scattering in Alkali-Earth Tungstate and Molybdate Crystals at Both Stretching and Bending Raman Modes under Synchronous Picosecond Pumping with Multiple Pulse Shortening Down to 1 ps |
title_short |
Stimulated Raman Scattering in Alkali-Earth Tungstate and Molybdate Crystals at Both Stretching and Bending Raman Modes under Synchronous Picosecond Pumping with Multiple Pulse Shortening Down to 1 ps |
title_full |
Stimulated Raman Scattering in Alkali-Earth Tungstate and Molybdate Crystals at Both Stretching and Bending Raman Modes under Synchronous Picosecond Pumping with Multiple Pulse Shortening Down to 1 ps |
title_fullStr |
Stimulated Raman Scattering in Alkali-Earth Tungstate and Molybdate Crystals at Both Stretching and Bending Raman Modes under Synchronous Picosecond Pumping with Multiple Pulse Shortening Down to 1 ps |
title_full_unstemmed |
Stimulated Raman Scattering in Alkali-Earth Tungstate and Molybdate Crystals at Both Stretching and Bending Raman Modes under Synchronous Picosecond Pumping with Multiple Pulse Shortening Down to 1 ps |
title_sort |
stimulated raman scattering in alkali-earth tungstate and molybdate crystals at both stretching and bending raman modes under synchronous picosecond pumping with multiple pulse shortening down to 1 ps |
publisher |
MDPI AG |
series |
Crystals |
issn |
2073-4352 |
publishDate |
2019-03-01 |
description |
Comparative investigation of characteristics of spontaneous and stimulated Raman scattering (SRS) in different alkali-earth tungstate and molybdate crystals at both high and low frequency anionic group vibrations is presented. It has been found that, among these crystals, the SrMoO<sub>4</sub> and SrWO<sub>4</sub> crystals are the most perspective for SRS generation on both stretching and bending modes of internal anionic group vibrations with the strongest SRS pulse shortening under synchronous laser pumping because of not only highly intense stretching mode Raman line for efficient primary extra cavity long-shifted SRS conversion but also the widest bending mode Raman line for the strongest SRS pulse shortening down to the inverse width of the widest Raman line (~1 ps) at secondary intracavity short-shifted SRS conversion. The strongest 26-fold pump pulse shortening down to 1.4 ps at the Stokes component with the combined Raman shift in the synchronously pumped extra cavity SrMoO<sub>4</sub> and SrWO<sub>4</sub> Raman lasers has been demonstrated. It was found that synchronously pumped cascade SRS with combined Raman shift is more efficient in the SrWO<sub>4</sub> crystal because the bending mode Raman line is more intense relative to the stretching mode Raman line than that in SrMoO<sub>4</sub>. |
topic |
alkali-earth tungstate molybdate crystals stretching bending Raman modes stimulated Raman scattering |
url |
https://www.mdpi.com/2073-4352/9/3/167 |
work_keys_str_mv |
AT milanfrank stimulatedramanscatteringinalkaliearthtungstateandmolybdatecrystalsatbothstretchingandbendingramanmodesundersynchronouspicosecondpumpingwithmultiplepulseshorteningdownto1ps AT sergeinsmetanin stimulatedramanscatteringinalkaliearthtungstateandmolybdatecrystalsatbothstretchingandbendingramanmodesundersynchronouspicosecondpumpingwithmultiplepulseshorteningdownto1ps AT michaljelinek stimulatedramanscatteringinalkaliearthtungstateandmolybdatecrystalsatbothstretchingandbendingramanmodesundersynchronouspicosecondpumpingwithmultiplepulseshorteningdownto1ps AT davidvyhlidal stimulatedramanscatteringinalkaliearthtungstateandmolybdatecrystalsatbothstretchingandbendingramanmodesundersynchronouspicosecondpumpingwithmultiplepulseshorteningdownto1ps AT vladislaveshukshin stimulatedramanscatteringinalkaliearthtungstateandmolybdatecrystalsatbothstretchingandbendingramanmodesundersynchronouspicosecondpumpingwithmultiplepulseshorteningdownto1ps AT lyudmilaiivleva stimulatedramanscatteringinalkaliearthtungstateandmolybdatecrystalsatbothstretchingandbendingramanmodesundersynchronouspicosecondpumpingwithmultiplepulseshorteningdownto1ps AT elizavetaedunaeva stimulatedramanscatteringinalkaliearthtungstateandmolybdatecrystalsatbothstretchingandbendingramanmodesundersynchronouspicosecondpumpingwithmultiplepulseshorteningdownto1ps AT irinasvoronina stimulatedramanscatteringinalkaliearthtungstateandmolybdatecrystalsatbothstretchingandbendingramanmodesundersynchronouspicosecondpumpingwithmultiplepulseshorteningdownto1ps AT petrgzverev stimulatedramanscatteringinalkaliearthtungstateandmolybdatecrystalsatbothstretchingandbendingramanmodesundersynchronouspicosecondpumpingwithmultiplepulseshorteningdownto1ps AT vaclavkubecek stimulatedramanscatteringinalkaliearthtungstateandmolybdatecrystalsatbothstretchingandbendingramanmodesundersynchronouspicosecondpumpingwithmultiplepulseshorteningdownto1ps |
_version_ |
1725805393785913344 |