Building and identifying highly active oxygenated groups in carbon materials for oxygen reduction to H2O2
The identity of catalytic sites for H2O2 generation in carbon-based materials remains controversial with limited experimental evidence to date. Here, the authors decorate various target functional groups on carbon materials and quinone-enriched samples exhibit the highest activity and selectivity.
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| Format: | Article |
| Language: | English |
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Nature Publishing Group
2020-05-01
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| Series: | Nature Communications |
| Online Access: | https://doi.org/10.1038/s41467-020-15782-z |
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doaj-8e3970b5411f43a084616a5641dde1b22021-05-11T09:04:39ZengNature Publishing GroupNature Communications2041-17232020-05-011111910.1038/s41467-020-15782-zBuilding and identifying highly active oxygenated groups in carbon materials for oxygen reduction to H2O2Gao-Feng Han0Feng Li1Wei Zou2Mohammadreza Karamad3Jong-Pil Jeon4Seong-Wook Kim5Seok-Jin Kim6Yunfei Bu7Zhengping Fu8Yalin Lu9Samira Siahrostami10Jong-Beom Baek11School of Energy and Chemical Engineering/Center for Dimension-Controllable Organic Frameworks, Ulsan National Institute of Science and Technology (UNIST)School of Energy and Chemical Engineering/Center for Dimension-Controllable Organic Frameworks, Ulsan National Institute of Science and Technology (UNIST)CAS Key Laboratory of Materials for Energy Conversion, Department of Materials Science and Engineering, University of Science and Technology of China (USTC)Department of Chemical and Petroleum Engineering, University of Calgary, 2500 University Drive NWSchool of Energy and Chemical Engineering/Center for Dimension-Controllable Organic Frameworks, Ulsan National Institute of Science and Technology (UNIST)School of Energy and Chemical Engineering/Center for Dimension-Controllable Organic Frameworks, Ulsan National Institute of Science and Technology (UNIST)School of Energy and Chemical Engineering/Center for Dimension-Controllable Organic Frameworks, Ulsan National Institute of Science and Technology (UNIST)Jiangsu Key Laboratory of Atmospheric Environment Monitoring and Pollution Control, School of Environmental Science and Engineering, Nanjing University of Information Science and Technology (NUIST), 219 NingliuCAS Key Laboratory of Materials for Energy Conversion, Department of Materials Science and Engineering, University of Science and Technology of China (USTC)CAS Key Laboratory of Materials for Energy Conversion, Department of Materials Science and Engineering, University of Science and Technology of China (USTC)Department of Chemistry, University of Calgary, 2500 University Drive NWSchool of Energy and Chemical Engineering/Center for Dimension-Controllable Organic Frameworks, Ulsan National Institute of Science and Technology (UNIST)The identity of catalytic sites for H2O2 generation in carbon-based materials remains controversial with limited experimental evidence to date. Here, the authors decorate various target functional groups on carbon materials and quinone-enriched samples exhibit the highest activity and selectivity.https://doi.org/10.1038/s41467-020-15782-z |
| collection |
DOAJ |
| language |
English |
| format |
Article |
| sources |
DOAJ |
| author |
Gao-Feng Han Feng Li Wei Zou Mohammadreza Karamad Jong-Pil Jeon Seong-Wook Kim Seok-Jin Kim Yunfei Bu Zhengping Fu Yalin Lu Samira Siahrostami Jong-Beom Baek |
| spellingShingle |
Gao-Feng Han Feng Li Wei Zou Mohammadreza Karamad Jong-Pil Jeon Seong-Wook Kim Seok-Jin Kim Yunfei Bu Zhengping Fu Yalin Lu Samira Siahrostami Jong-Beom Baek Building and identifying highly active oxygenated groups in carbon materials for oxygen reduction to H2O2 Nature Communications |
| author_facet |
Gao-Feng Han Feng Li Wei Zou Mohammadreza Karamad Jong-Pil Jeon Seong-Wook Kim Seok-Jin Kim Yunfei Bu Zhengping Fu Yalin Lu Samira Siahrostami Jong-Beom Baek |
| author_sort |
Gao-Feng Han |
| title |
Building and identifying highly active oxygenated groups in carbon materials for oxygen reduction to H2O2 |
| title_short |
Building and identifying highly active oxygenated groups in carbon materials for oxygen reduction to H2O2 |
| title_full |
Building and identifying highly active oxygenated groups in carbon materials for oxygen reduction to H2O2 |
| title_fullStr |
Building and identifying highly active oxygenated groups in carbon materials for oxygen reduction to H2O2 |
| title_full_unstemmed |
Building and identifying highly active oxygenated groups in carbon materials for oxygen reduction to H2O2 |
| title_sort |
building and identifying highly active oxygenated groups in carbon materials for oxygen reduction to h2o2 |
| publisher |
Nature Publishing Group |
| series |
Nature Communications |
| issn |
2041-1723 |
| publishDate |
2020-05-01 |
| description |
The identity of catalytic sites for H2O2 generation in carbon-based materials remains controversial with limited experimental evidence to date. Here, the authors decorate various target functional groups on carbon materials and quinone-enriched samples exhibit the highest activity and selectivity. |
| url |
https://doi.org/10.1038/s41467-020-15782-z |
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