TiO<sub>2</sub> Nanowires with Doped g-C<sub>3</sub>N<sub>4</sub> Nanoparticles for Enhanced H<sub>2</sub> Production and Photodegradation of Pollutants
With the rapid consumption of fossil fuels, along with the ever-increasing environmental pollution, it is becoming a top priority to explore efficient photocatalysts for the production of renewable hydrogen and degradation of pollutants. Here, we fabricated a composite of g-C<sub>3</sub>...
Main Authors: | , , , , , , , , , , |
---|---|
Format: | Article |
Language: | English |
Published: |
MDPI AG
2021-01-01
|
Series: | Nanomaterials |
Subjects: | |
Online Access: | https://www.mdpi.com/2079-4991/11/1/254 |
id |
doaj-94e1ac3ca7db48edb83f4dc61f3f3a9b |
---|---|
record_format |
Article |
spelling |
doaj-94e1ac3ca7db48edb83f4dc61f3f3a9b2021-01-20T00:04:38ZengMDPI AGNanomaterials2079-49912021-01-011125425410.3390/nano11010254TiO<sub>2</sub> Nanowires with Doped g-C<sub>3</sub>N<sub>4</sub> Nanoparticles for Enhanced H<sub>2</sub> Production and Photodegradation of PollutantsLiushan Jiang0Fanshan Zeng1Rong Zhong2Yu Xie3Jianli Wang4Hao Ye5Yun Ling6Ruobin Guo7Jinsheng Zhao8Shiqian Li9Yuying Hu10College of Environment and Chemical Engineering, Nanchang Hangkong University, Nanchang 330063, ChinaCollege of Environment and Chemical Engineering, Nanchang Hangkong University, Nanchang 330063, ChinaCollege of Environment and Chemical Engineering, Nanchang Hangkong University, Nanchang 330063, ChinaCollege of Environment and Chemical Engineering, Nanchang Hangkong University, Nanchang 330063, ChinaCollege of Environment and Chemical Engineering, Nanchang Hangkong University, Nanchang 330063, ChinaCollege of Environment and Chemical Engineering, Nanchang Hangkong University, Nanchang 330063, ChinaCollege of Environment and Chemical Engineering, Nanchang Hangkong University, Nanchang 330063, ChinaCollege of Environment and Chemical Engineering, Nanchang Hangkong University, Nanchang 330063, ChinaShandong Key Laboratory of Chemical Energy Storage and Novel Cell Technology, Liaocheng University, Liaocheng 252059, ChinaSchool of Ocean Science and Biochemistry Engineering, Fuqing Branch of Fujian Normal University, Fuqing 350300, ChinaSchool of Civil Engineering and Architecture, East China Jiaotong University, Nanchang 330013, ChinaWith the rapid consumption of fossil fuels, along with the ever-increasing environmental pollution, it is becoming a top priority to explore efficient photocatalysts for the production of renewable hydrogen and degradation of pollutants. Here, we fabricated a composite of g-C<sub>3</sub>N<sub>4</sub>/TiO<sub>2</sub> via an in situ growth method under the conditions of high-temperature calcination. In this method, TiO<sub>2</sub> nanowires with a large specific surface area could provide enough space for loading more g-C<sub>3</sub>N<sub>4</sub> nanoparticles to obtain C<sub>3</sub>N<sub>4</sub>/TiO<sub>2 </sub>composites. Of note, the g-C<sub>3</sub>N<sub>4</sub>/TiO<sub>2 </sub>composite could effectively photocatalyze both the degradation of several pollutants and production of hydrogen, both of which are essential for environmental governance. Combining multiple characterizations and experiments, we found that the heterojunction constructed by the TiO<sub>2 </sub>and g-C<sub>3</sub>N<sub>4</sub> could increase the photocatalytic ability of materials by prompting the separation of photogenerated carriers. Furthermore, the photocatalytic mechanism of the g-C<sub>3</sub>N<sub>4</sub>/TiO<sub>2 </sub>composite was also clarified in detail.https://www.mdpi.com/2079-4991/11/1/254TiO<sub>2</sub> nanowireg-C<sub>3</sub>N<sub>4</sub> particlesg-C<sub>3</sub>N<sub>4</sub>/TiO<sub>2</sub> compositephotodegradation of pollutants |
collection |
DOAJ |
language |
English |
format |
Article |
sources |
DOAJ |
author |
Liushan Jiang Fanshan Zeng Rong Zhong Yu Xie Jianli Wang Hao Ye Yun Ling Ruobin Guo Jinsheng Zhao Shiqian Li Yuying Hu |
spellingShingle |
Liushan Jiang Fanshan Zeng Rong Zhong Yu Xie Jianli Wang Hao Ye Yun Ling Ruobin Guo Jinsheng Zhao Shiqian Li Yuying Hu TiO<sub>2</sub> Nanowires with Doped g-C<sub>3</sub>N<sub>4</sub> Nanoparticles for Enhanced H<sub>2</sub> Production and Photodegradation of Pollutants Nanomaterials TiO<sub>2</sub> nanowire g-C<sub>3</sub>N<sub>4</sub> particles g-C<sub>3</sub>N<sub>4</sub>/TiO<sub>2</sub> composite photodegradation of pollutants |
author_facet |
Liushan Jiang Fanshan Zeng Rong Zhong Yu Xie Jianli Wang Hao Ye Yun Ling Ruobin Guo Jinsheng Zhao Shiqian Li Yuying Hu |
author_sort |
Liushan Jiang |
title |
TiO<sub>2</sub> Nanowires with Doped g-C<sub>3</sub>N<sub>4</sub> Nanoparticles for Enhanced H<sub>2</sub> Production and Photodegradation of Pollutants |
title_short |
TiO<sub>2</sub> Nanowires with Doped g-C<sub>3</sub>N<sub>4</sub> Nanoparticles for Enhanced H<sub>2</sub> Production and Photodegradation of Pollutants |
title_full |
TiO<sub>2</sub> Nanowires with Doped g-C<sub>3</sub>N<sub>4</sub> Nanoparticles for Enhanced H<sub>2</sub> Production and Photodegradation of Pollutants |
title_fullStr |
TiO<sub>2</sub> Nanowires with Doped g-C<sub>3</sub>N<sub>4</sub> Nanoparticles for Enhanced H<sub>2</sub> Production and Photodegradation of Pollutants |
title_full_unstemmed |
TiO<sub>2</sub> Nanowires with Doped g-C<sub>3</sub>N<sub>4</sub> Nanoparticles for Enhanced H<sub>2</sub> Production and Photodegradation of Pollutants |
title_sort |
tio<sub>2</sub> nanowires with doped g-c<sub>3</sub>n<sub>4</sub> nanoparticles for enhanced h<sub>2</sub> production and photodegradation of pollutants |
publisher |
MDPI AG |
series |
Nanomaterials |
issn |
2079-4991 |
publishDate |
2021-01-01 |
description |
With the rapid consumption of fossil fuels, along with the ever-increasing environmental pollution, it is becoming a top priority to explore efficient photocatalysts for the production of renewable hydrogen and degradation of pollutants. Here, we fabricated a composite of g-C<sub>3</sub>N<sub>4</sub>/TiO<sub>2</sub> via an in situ growth method under the conditions of high-temperature calcination. In this method, TiO<sub>2</sub> nanowires with a large specific surface area could provide enough space for loading more g-C<sub>3</sub>N<sub>4</sub> nanoparticles to obtain C<sub>3</sub>N<sub>4</sub>/TiO<sub>2 </sub>composites. Of note, the g-C<sub>3</sub>N<sub>4</sub>/TiO<sub>2 </sub>composite could effectively photocatalyze both the degradation of several pollutants and production of hydrogen, both of which are essential for environmental governance. Combining multiple characterizations and experiments, we found that the heterojunction constructed by the TiO<sub>2 </sub>and g-C<sub>3</sub>N<sub>4</sub> could increase the photocatalytic ability of materials by prompting the separation of photogenerated carriers. Furthermore, the photocatalytic mechanism of the g-C<sub>3</sub>N<sub>4</sub>/TiO<sub>2 </sub>composite was also clarified in detail. |
topic |
TiO<sub>2</sub> nanowire g-C<sub>3</sub>N<sub>4</sub> particles g-C<sub>3</sub>N<sub>4</sub>/TiO<sub>2</sub> composite photodegradation of pollutants |
url |
https://www.mdpi.com/2079-4991/11/1/254 |
work_keys_str_mv |
AT liushanjiang tiosub2subnanowireswithdopedgcsub3subnsub4subnanoparticlesforenhancedhsub2subproductionandphotodegradationofpollutants AT fanshanzeng tiosub2subnanowireswithdopedgcsub3subnsub4subnanoparticlesforenhancedhsub2subproductionandphotodegradationofpollutants AT rongzhong tiosub2subnanowireswithdopedgcsub3subnsub4subnanoparticlesforenhancedhsub2subproductionandphotodegradationofpollutants AT yuxie tiosub2subnanowireswithdopedgcsub3subnsub4subnanoparticlesforenhancedhsub2subproductionandphotodegradationofpollutants AT jianliwang tiosub2subnanowireswithdopedgcsub3subnsub4subnanoparticlesforenhancedhsub2subproductionandphotodegradationofpollutants AT haoye tiosub2subnanowireswithdopedgcsub3subnsub4subnanoparticlesforenhancedhsub2subproductionandphotodegradationofpollutants AT yunling tiosub2subnanowireswithdopedgcsub3subnsub4subnanoparticlesforenhancedhsub2subproductionandphotodegradationofpollutants AT ruobinguo tiosub2subnanowireswithdopedgcsub3subnsub4subnanoparticlesforenhancedhsub2subproductionandphotodegradationofpollutants AT jinshengzhao tiosub2subnanowireswithdopedgcsub3subnsub4subnanoparticlesforenhancedhsub2subproductionandphotodegradationofpollutants AT shiqianli tiosub2subnanowireswithdopedgcsub3subnsub4subnanoparticlesforenhancedhsub2subproductionandphotodegradationofpollutants AT yuyinghu tiosub2subnanowireswithdopedgcsub3subnsub4subnanoparticlesforenhancedhsub2subproductionandphotodegradationofpollutants |
_version_ |
1724331499070685184 |