TiO<sub>2</sub> Nanowires with Doped g-C<sub>3</sub>N<sub>4</sub> Nanoparticles for Enhanced H<sub>2</sub> Production and Photodegradation of Pollutants

With the rapid consumption of fossil fuels, along with the ever-increasing environmental pollution, it is becoming a top priority to explore efficient photocatalysts for the production of renewable hydrogen and degradation of pollutants. Here, we fabricated a composite of g-C<sub>3</sub>...

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Main Authors: Liushan Jiang, Fanshan Zeng, Rong Zhong, Yu Xie, Jianli Wang, Hao Ye, Yun Ling, Ruobin Guo, Jinsheng Zhao, Shiqian Li, Yuying Hu
Format: Article
Language:English
Published: MDPI AG 2021-01-01
Series:Nanomaterials
Subjects:
Online Access:https://www.mdpi.com/2079-4991/11/1/254
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spelling doaj-94e1ac3ca7db48edb83f4dc61f3f3a9b2021-01-20T00:04:38ZengMDPI AGNanomaterials2079-49912021-01-011125425410.3390/nano11010254TiO<sub>2</sub> Nanowires with Doped g-C<sub>3</sub>N<sub>4</sub> Nanoparticles for Enhanced H<sub>2</sub> Production and Photodegradation of PollutantsLiushan Jiang0Fanshan Zeng1Rong Zhong2Yu Xie3Jianli Wang4Hao Ye5Yun Ling6Ruobin Guo7Jinsheng Zhao8Shiqian Li9Yuying Hu10College of Environment and Chemical Engineering, Nanchang Hangkong University, Nanchang 330063, ChinaCollege of Environment and Chemical Engineering, Nanchang Hangkong University, Nanchang 330063, ChinaCollege of Environment and Chemical Engineering, Nanchang Hangkong University, Nanchang 330063, ChinaCollege of Environment and Chemical Engineering, Nanchang Hangkong University, Nanchang 330063, ChinaCollege of Environment and Chemical Engineering, Nanchang Hangkong University, Nanchang 330063, ChinaCollege of Environment and Chemical Engineering, Nanchang Hangkong University, Nanchang 330063, ChinaCollege of Environment and Chemical Engineering, Nanchang Hangkong University, Nanchang 330063, ChinaCollege of Environment and Chemical Engineering, Nanchang Hangkong University, Nanchang 330063, ChinaShandong Key Laboratory of Chemical Energy Storage and Novel Cell Technology, Liaocheng University, Liaocheng 252059, ChinaSchool of Ocean Science and Biochemistry Engineering, Fuqing Branch of Fujian Normal University, Fuqing 350300, ChinaSchool of Civil Engineering and Architecture, East China Jiaotong University, Nanchang 330013, ChinaWith the rapid consumption of fossil fuels, along with the ever-increasing environmental pollution, it is becoming a top priority to explore efficient photocatalysts for the production of renewable hydrogen and degradation of pollutants. Here, we fabricated a composite of g-C<sub>3</sub>N<sub>4</sub>/TiO<sub>2</sub> via an in situ growth method under the conditions of high-temperature calcination. In this method, TiO<sub>2</sub> nanowires with a large specific surface area could provide enough space for loading more g-C<sub>3</sub>N<sub>4</sub> nanoparticles to obtain C<sub>3</sub>N<sub>4</sub>/TiO<sub>2 </sub>composites. Of note, the g-C<sub>3</sub>N<sub>4</sub>/TiO<sub>2 </sub>composite could effectively photocatalyze both the degradation of several pollutants and production of hydrogen, both of which are essential for environmental governance. Combining multiple characterizations and experiments, we found that the heterojunction constructed by the TiO<sub>2 </sub>and g-C<sub>3</sub>N<sub>4</sub> could increase the photocatalytic ability of materials by prompting the separation of photogenerated carriers. Furthermore, the photocatalytic mechanism of the g-C<sub>3</sub>N<sub>4</sub>/TiO<sub>2 </sub>composite was also clarified in detail.https://www.mdpi.com/2079-4991/11/1/254TiO<sub>2</sub> nanowireg-C<sub>3</sub>N<sub>4</sub> particlesg-C<sub>3</sub>N<sub>4</sub>/TiO<sub>2</sub> compositephotodegradation of pollutants
collection DOAJ
language English
format Article
sources DOAJ
author Liushan Jiang
Fanshan Zeng
Rong Zhong
Yu Xie
Jianli Wang
Hao Ye
Yun Ling
Ruobin Guo
Jinsheng Zhao
Shiqian Li
Yuying Hu
spellingShingle Liushan Jiang
Fanshan Zeng
Rong Zhong
Yu Xie
Jianli Wang
Hao Ye
Yun Ling
Ruobin Guo
Jinsheng Zhao
Shiqian Li
Yuying Hu
TiO<sub>2</sub> Nanowires with Doped g-C<sub>3</sub>N<sub>4</sub> Nanoparticles for Enhanced H<sub>2</sub> Production and Photodegradation of Pollutants
Nanomaterials
TiO<sub>2</sub> nanowire
g-C<sub>3</sub>N<sub>4</sub> particles
g-C<sub>3</sub>N<sub>4</sub>/TiO<sub>2</sub> composite
photodegradation of pollutants
author_facet Liushan Jiang
Fanshan Zeng
Rong Zhong
Yu Xie
Jianli Wang
Hao Ye
Yun Ling
Ruobin Guo
Jinsheng Zhao
Shiqian Li
Yuying Hu
author_sort Liushan Jiang
title TiO<sub>2</sub> Nanowires with Doped g-C<sub>3</sub>N<sub>4</sub> Nanoparticles for Enhanced H<sub>2</sub> Production and Photodegradation of Pollutants
title_short TiO<sub>2</sub> Nanowires with Doped g-C<sub>3</sub>N<sub>4</sub> Nanoparticles for Enhanced H<sub>2</sub> Production and Photodegradation of Pollutants
title_full TiO<sub>2</sub> Nanowires with Doped g-C<sub>3</sub>N<sub>4</sub> Nanoparticles for Enhanced H<sub>2</sub> Production and Photodegradation of Pollutants
title_fullStr TiO<sub>2</sub> Nanowires with Doped g-C<sub>3</sub>N<sub>4</sub> Nanoparticles for Enhanced H<sub>2</sub> Production and Photodegradation of Pollutants
title_full_unstemmed TiO<sub>2</sub> Nanowires with Doped g-C<sub>3</sub>N<sub>4</sub> Nanoparticles for Enhanced H<sub>2</sub> Production and Photodegradation of Pollutants
title_sort tio<sub>2</sub> nanowires with doped g-c<sub>3</sub>n<sub>4</sub> nanoparticles for enhanced h<sub>2</sub> production and photodegradation of pollutants
publisher MDPI AG
series Nanomaterials
issn 2079-4991
publishDate 2021-01-01
description With the rapid consumption of fossil fuels, along with the ever-increasing environmental pollution, it is becoming a top priority to explore efficient photocatalysts for the production of renewable hydrogen and degradation of pollutants. Here, we fabricated a composite of g-C<sub>3</sub>N<sub>4</sub>/TiO<sub>2</sub> via an in situ growth method under the conditions of high-temperature calcination. In this method, TiO<sub>2</sub> nanowires with a large specific surface area could provide enough space for loading more g-C<sub>3</sub>N<sub>4</sub> nanoparticles to obtain C<sub>3</sub>N<sub>4</sub>/TiO<sub>2 </sub>composites. Of note, the g-C<sub>3</sub>N<sub>4</sub>/TiO<sub>2 </sub>composite could effectively photocatalyze both the degradation of several pollutants and production of hydrogen, both of which are essential for environmental governance. Combining multiple characterizations and experiments, we found that the heterojunction constructed by the TiO<sub>2 </sub>and g-C<sub>3</sub>N<sub>4</sub> could increase the photocatalytic ability of materials by prompting the separation of photogenerated carriers. Furthermore, the photocatalytic mechanism of the g-C<sub>3</sub>N<sub>4</sub>/TiO<sub>2 </sub>composite was also clarified in detail.
topic TiO<sub>2</sub> nanowire
g-C<sub>3</sub>N<sub>4</sub> particles
g-C<sub>3</sub>N<sub>4</sub>/TiO<sub>2</sub> composite
photodegradation of pollutants
url https://www.mdpi.com/2079-4991/11/1/254
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