Demystifying the growth of superconducting Sr2RuO4 thin films

We report the growth of superconducting Sr2RuO4 thin films by molecular-beam epitaxy on (110) NdGaO3 substrates with transition temperatures of up to 1.8 K. We calculate and experimentally validate a thermodynamic growth window for the adsorption-controlled growth of superconducting Sr2RuO4 epitaxia...

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Main Authors: Hari P. Nair, Jacob P. Ruf, Nathaniel J. Schreiber, Ludi Miao, Morgan L. Grandon, David J. Baek, Berit H. Goodge, Jacob P. C. Ruff, Lena F. Kourkoutis, Kyle M. Shen, Darrell G. Schlom
Format: Article
Language:English
Published: AIP Publishing LLC 2018-10-01
Series:APL Materials
Online Access:http://dx.doi.org/10.1063/1.5053084
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spelling doaj-9d7ba77f20f04fe0b7f550b025142bf42020-11-24T21:49:51ZengAIP Publishing LLCAPL Materials2166-532X2018-10-01610101108101108-810.1063/1.5053084011810APMDemystifying the growth of superconducting Sr2RuO4 thin filmsHari P. Nair0Jacob P. Ruf1Nathaniel J. Schreiber2Ludi Miao3Morgan L. Grandon4David J. Baek5Berit H. Goodge6Jacob P. C. Ruff7Lena F. Kourkoutis8Kyle M. Shen9Darrell G. Schlom10Department of Materials Science and Engineering, Cornell University, Ithaca, New York 14853, USADepartment of Physics, Cornell University, Ithaca, New York 14853, USADepartment of Materials Science and Engineering, Cornell University, Ithaca, New York 14853, USADepartment of Physics, Cornell University, Ithaca, New York 14853, USADepartment of Materials Science and Engineering, Cornell University, Ithaca, New York 14853, USASchool of Electrical and Computer Engineering, Cornell University, Ithaca, New York 14853, USASchool of Applied and Engineering Physics, Cornell University, Ithaca, New York 14853, USACornell High Energy Synchrotron Source, Cornell University, Ithaca, New York 14853, USASchool of Applied and Engineering Physics, Cornell University, Ithaca, New York 14853, USADepartment of Physics, Cornell University, Ithaca, New York 14853, USADepartment of Materials Science and Engineering, Cornell University, Ithaca, New York 14853, USAWe report the growth of superconducting Sr2RuO4 thin films by molecular-beam epitaxy on (110) NdGaO3 substrates with transition temperatures of up to 1.8 K. We calculate and experimentally validate a thermodynamic growth window for the adsorption-controlled growth of superconducting Sr2RuO4 epitaxial thin films. The growth window for achieving superconducting Sr2RuO4 thin films is narrow in growth temperature, oxidant pressure, and ruthenium-to-strontium flux ratio.http://dx.doi.org/10.1063/1.5053084
collection DOAJ
language English
format Article
sources DOAJ
author Hari P. Nair
Jacob P. Ruf
Nathaniel J. Schreiber
Ludi Miao
Morgan L. Grandon
David J. Baek
Berit H. Goodge
Jacob P. C. Ruff
Lena F. Kourkoutis
Kyle M. Shen
Darrell G. Schlom
spellingShingle Hari P. Nair
Jacob P. Ruf
Nathaniel J. Schreiber
Ludi Miao
Morgan L. Grandon
David J. Baek
Berit H. Goodge
Jacob P. C. Ruff
Lena F. Kourkoutis
Kyle M. Shen
Darrell G. Schlom
Demystifying the growth of superconducting Sr2RuO4 thin films
APL Materials
author_facet Hari P. Nair
Jacob P. Ruf
Nathaniel J. Schreiber
Ludi Miao
Morgan L. Grandon
David J. Baek
Berit H. Goodge
Jacob P. C. Ruff
Lena F. Kourkoutis
Kyle M. Shen
Darrell G. Schlom
author_sort Hari P. Nair
title Demystifying the growth of superconducting Sr2RuO4 thin films
title_short Demystifying the growth of superconducting Sr2RuO4 thin films
title_full Demystifying the growth of superconducting Sr2RuO4 thin films
title_fullStr Demystifying the growth of superconducting Sr2RuO4 thin films
title_full_unstemmed Demystifying the growth of superconducting Sr2RuO4 thin films
title_sort demystifying the growth of superconducting sr2ruo4 thin films
publisher AIP Publishing LLC
series APL Materials
issn 2166-532X
publishDate 2018-10-01
description We report the growth of superconducting Sr2RuO4 thin films by molecular-beam epitaxy on (110) NdGaO3 substrates with transition temperatures of up to 1.8 K. We calculate and experimentally validate a thermodynamic growth window for the adsorption-controlled growth of superconducting Sr2RuO4 epitaxial thin films. The growth window for achieving superconducting Sr2RuO4 thin films is narrow in growth temperature, oxidant pressure, and ruthenium-to-strontium flux ratio.
url http://dx.doi.org/10.1063/1.5053084
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