Interfacial engineering of metal-insulator-semiconductor junctions for efficient and stable photoelectrochemical water oxidation

Solar water splitting using metal–insulator–semiconductor junctions has proven efficient, but these junctions degrade very rapidly. Here, the authors engineer metal–insulator–semiconductor interfaces in which Fermi-level pinning is reduced, producing an efficient and durable photoanode for solar-dri...

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Main Authors:	Ibadillah A. Digdaya, Gede W. P. Adhyaksa, Bartek J. Trześniewski, Erik C. Garnett, Wilson A. Smith
Format:	Article
Language:	English
Published:	Nature Publishing Group 2017-06-01
Series:	Nature Communications
Online Access:	https://doi.org/10.1038/ncomms15968

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spelling	doaj-9d949616628447d7ac74ea436a6332062021-05-11T07:22:28ZengNature Publishing GroupNature Communications2041-17232017-06-01811810.1038/ncomms15968Interfacial engineering of metal-insulator-semiconductor junctions for efficient and stable photoelectrochemical water oxidationIbadillah A. Digdaya0Gede W. P. Adhyaksa1Bartek J. Trześniewski2Erik C. Garnett3Wilson A. Smith4Department of Chemical Engineering, Materials for Energy Conversion and Storage (MECS), Delft University of TechnologyCenter for Nanophotonics, AMOLFDepartment of Chemical Engineering, Materials for Energy Conversion and Storage (MECS), Delft University of TechnologyCenter for Nanophotonics, AMOLFDepartment of Chemical Engineering, Materials for Energy Conversion and Storage (MECS), Delft University of TechnologySolar water splitting using metal–insulator–semiconductor junctions has proven efficient, but these junctions degrade very rapidly. Here, the authors engineer metal–insulator–semiconductor interfaces in which Fermi-level pinning is reduced, producing an efficient and durable photoanode for solar-driven water oxidation.https://doi.org/10.1038/ncomms15968
collection	DOAJ
language	English
format	Article
sources	DOAJ
author	Ibadillah A. Digdaya Gede W. P. Adhyaksa Bartek J. Trześniewski Erik C. Garnett Wilson A. Smith
spellingShingle	Ibadillah A. Digdaya Gede W. P. Adhyaksa Bartek J. Trześniewski Erik C. Garnett Wilson A. Smith Interfacial engineering of metal-insulator-semiconductor junctions for efficient and stable photoelectrochemical water oxidation Nature Communications
author_facet	Ibadillah A. Digdaya Gede W. P. Adhyaksa Bartek J. Trześniewski Erik C. Garnett Wilson A. Smith
author_sort	Ibadillah A. Digdaya
title	Interfacial engineering of metal-insulator-semiconductor junctions for efficient and stable photoelectrochemical water oxidation
title_short	Interfacial engineering of metal-insulator-semiconductor junctions for efficient and stable photoelectrochemical water oxidation
title_full	Interfacial engineering of metal-insulator-semiconductor junctions for efficient and stable photoelectrochemical water oxidation
title_fullStr	Interfacial engineering of metal-insulator-semiconductor junctions for efficient and stable photoelectrochemical water oxidation
title_full_unstemmed	Interfacial engineering of metal-insulator-semiconductor junctions for efficient and stable photoelectrochemical water oxidation
title_sort	interfacial engineering of metal-insulator-semiconductor junctions for efficient and stable photoelectrochemical water oxidation
publisher	Nature Publishing Group
series	Nature Communications
issn	2041-1723
publishDate	2017-06-01
description	Solar water splitting using metal–insulator–semiconductor junctions has proven efficient, but these junctions degrade very rapidly. Here, the authors engineer metal–insulator–semiconductor interfaces in which Fermi-level pinning is reduced, producing an efficient and durable photoanode for solar-driven water oxidation.
url	https://doi.org/10.1038/ncomms15968
work_keys_str_mv	AT ibadillahadigdaya interfacialengineeringofmetalinsulatorsemiconductorjunctionsforefficientandstablephotoelectrochemicalwateroxidation AT gedewpadhyaksa interfacialengineeringofmetalinsulatorsemiconductorjunctionsforefficientandstablephotoelectrochemicalwateroxidation AT bartekjtrzesniewski interfacialengineeringofmetalinsulatorsemiconductorjunctionsforefficientandstablephotoelectrochemicalwateroxidation AT erikcgarnett interfacialengineeringofmetalinsulatorsemiconductorjunctionsforefficientandstablephotoelectrochemicalwateroxidation AT wilsonasmith interfacialengineeringofmetalinsulatorsemiconductorjunctionsforefficientandstablephotoelectrochemicalwateroxidation
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Interfacial engineering of metal-insulator-semiconductor junctions for efficient and stable photoelectrochemical water oxidation

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