Combined Nanofiltration and Thermocatalysis for the Simultaneous Degradation of Micropollutants, Fouling Mitigation and Water Purification

Due to progressive limitation of access to clean drinkable water, it is nowadays a priority to find an effective method of water purification from those emerging organic contaminants, which might have potentially harmful and irreversible effects on living organisms and environment. This manuscript r...

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Main Authors: Katarzyna Janowska, Xianzheng Ma, Vittorio Boffa, Mads Koustrup Jørgensen, Victor M. Candelario
Format: Article
Language:English
Published: MDPI AG 2021-08-01
Series:Membranes
Subjects:
Online Access:https://www.mdpi.com/2077-0375/11/8/639
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spelling doaj-a162b3fde48b4a46aef1a1000ca85aa32021-08-26T14:03:34ZengMDPI AGMembranes2077-03752021-08-011163963910.3390/membranes11080639Combined Nanofiltration and Thermocatalysis for the Simultaneous Degradation of Micropollutants, Fouling Mitigation and Water PurificationKatarzyna Janowska0Xianzheng Ma1Vittorio Boffa2Mads Koustrup Jørgensen3Victor M. Candelario4Center for Membrane Technology, Department of Chemistry and Bioscience, Aalborg University, Fredrik Bajers Vej 7H, 9220 Aalborg, DenmarkCenter for Membrane Technology, Department of Chemistry and Bioscience, Aalborg University, Fredrik Bajers Vej 7H, 9220 Aalborg, DenmarkCenter for Membrane Technology, Department of Chemistry and Bioscience, Aalborg University, Fredrik Bajers Vej 7H, 9220 Aalborg, DenmarkCenter for Membrane Technology, Department of Chemistry and Bioscience, Aalborg University, Fredrik Bajers Vej 7H, 9220 Aalborg, DenmarkDepartment of Research and Development, LiqTech Ceramics A/S, Industriparken 22C, 2750 Ballerup, DenmarkDue to progressive limitation of access to clean drinkable water, it is nowadays a priority to find an effective method of water purification from those emerging organic contaminants, which might have potentially harmful and irreversible effects on living organisms and environment. This manuscript reports the development of a new strategy for water purification, which combines a novel and recently developed Al<sub>2</sub>O<sub>3</sub>-doped silica nanofiltration membrane with a thermocatalytic perovskite, namely cerium-doped strontium ferrate (CSF). The thermocatalytic activity of CSF offers the opportunity to degrade organic pollutants with no light and without input of chemical oxidants, providing simplicity of operation. Moreover, our studies on real samples of secondary effluent from wastewater treatment showed that the thermocatalyst has the ability to degrade also part of the non-toxic organic matter, which allows for reducing the chemical oxygen demand of the retentate and mitigating membrane fouling during filtration. Therefore, the new technology is effective in the production of clean feed and permeate and has a potential to be used in degradation of micropollutants in water treatment.https://www.mdpi.com/2077-0375/11/8/639nanofiltrationthermocatalysisperovskitemicropollutantswater purificationwastewater
collection DOAJ
language English
format Article
sources DOAJ
author Katarzyna Janowska
Xianzheng Ma
Vittorio Boffa
Mads Koustrup Jørgensen
Victor M. Candelario
spellingShingle Katarzyna Janowska
Xianzheng Ma
Vittorio Boffa
Mads Koustrup Jørgensen
Victor M. Candelario
Combined Nanofiltration and Thermocatalysis for the Simultaneous Degradation of Micropollutants, Fouling Mitigation and Water Purification
Membranes
nanofiltration
thermocatalysis
perovskite
micropollutants
water purification
wastewater
author_facet Katarzyna Janowska
Xianzheng Ma
Vittorio Boffa
Mads Koustrup Jørgensen
Victor M. Candelario
author_sort Katarzyna Janowska
title Combined Nanofiltration and Thermocatalysis for the Simultaneous Degradation of Micropollutants, Fouling Mitigation and Water Purification
title_short Combined Nanofiltration and Thermocatalysis for the Simultaneous Degradation of Micropollutants, Fouling Mitigation and Water Purification
title_full Combined Nanofiltration and Thermocatalysis for the Simultaneous Degradation of Micropollutants, Fouling Mitigation and Water Purification
title_fullStr Combined Nanofiltration and Thermocatalysis for the Simultaneous Degradation of Micropollutants, Fouling Mitigation and Water Purification
title_full_unstemmed Combined Nanofiltration and Thermocatalysis for the Simultaneous Degradation of Micropollutants, Fouling Mitigation and Water Purification
title_sort combined nanofiltration and thermocatalysis for the simultaneous degradation of micropollutants, fouling mitigation and water purification
publisher MDPI AG
series Membranes
issn 2077-0375
publishDate 2021-08-01
description Due to progressive limitation of access to clean drinkable water, it is nowadays a priority to find an effective method of water purification from those emerging organic contaminants, which might have potentially harmful and irreversible effects on living organisms and environment. This manuscript reports the development of a new strategy for water purification, which combines a novel and recently developed Al<sub>2</sub>O<sub>3</sub>-doped silica nanofiltration membrane with a thermocatalytic perovskite, namely cerium-doped strontium ferrate (CSF). The thermocatalytic activity of CSF offers the opportunity to degrade organic pollutants with no light and without input of chemical oxidants, providing simplicity of operation. Moreover, our studies on real samples of secondary effluent from wastewater treatment showed that the thermocatalyst has the ability to degrade also part of the non-toxic organic matter, which allows for reducing the chemical oxygen demand of the retentate and mitigating membrane fouling during filtration. Therefore, the new technology is effective in the production of clean feed and permeate and has a potential to be used in degradation of micropollutants in water treatment.
topic nanofiltration
thermocatalysis
perovskite
micropollutants
water purification
wastewater
url https://www.mdpi.com/2077-0375/11/8/639
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AT xianzhengma combinednanofiltrationandthermocatalysisforthesimultaneousdegradationofmicropollutantsfoulingmitigationandwaterpurification
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