Combined Nanofiltration and Thermocatalysis for the Simultaneous Degradation of Micropollutants, Fouling Mitigation and Water Purification
Due to progressive limitation of access to clean drinkable water, it is nowadays a priority to find an effective method of water purification from those emerging organic contaminants, which might have potentially harmful and irreversible effects on living organisms and environment. This manuscript r...
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doaj-a162b3fde48b4a46aef1a1000ca85aa32021-08-26T14:03:34ZengMDPI AGMembranes2077-03752021-08-011163963910.3390/membranes11080639Combined Nanofiltration and Thermocatalysis for the Simultaneous Degradation of Micropollutants, Fouling Mitigation and Water PurificationKatarzyna Janowska0Xianzheng Ma1Vittorio Boffa2Mads Koustrup Jørgensen3Victor M. Candelario4Center for Membrane Technology, Department of Chemistry and Bioscience, Aalborg University, Fredrik Bajers Vej 7H, 9220 Aalborg, DenmarkCenter for Membrane Technology, Department of Chemistry and Bioscience, Aalborg University, Fredrik Bajers Vej 7H, 9220 Aalborg, DenmarkCenter for Membrane Technology, Department of Chemistry and Bioscience, Aalborg University, Fredrik Bajers Vej 7H, 9220 Aalborg, DenmarkCenter for Membrane Technology, Department of Chemistry and Bioscience, Aalborg University, Fredrik Bajers Vej 7H, 9220 Aalborg, DenmarkDepartment of Research and Development, LiqTech Ceramics A/S, Industriparken 22C, 2750 Ballerup, DenmarkDue to progressive limitation of access to clean drinkable water, it is nowadays a priority to find an effective method of water purification from those emerging organic contaminants, which might have potentially harmful and irreversible effects on living organisms and environment. This manuscript reports the development of a new strategy for water purification, which combines a novel and recently developed Al<sub>2</sub>O<sub>3</sub>-doped silica nanofiltration membrane with a thermocatalytic perovskite, namely cerium-doped strontium ferrate (CSF). The thermocatalytic activity of CSF offers the opportunity to degrade organic pollutants with no light and without input of chemical oxidants, providing simplicity of operation. Moreover, our studies on real samples of secondary effluent from wastewater treatment showed that the thermocatalyst has the ability to degrade also part of the non-toxic organic matter, which allows for reducing the chemical oxygen demand of the retentate and mitigating membrane fouling during filtration. Therefore, the new technology is effective in the production of clean feed and permeate and has a potential to be used in degradation of micropollutants in water treatment.https://www.mdpi.com/2077-0375/11/8/639nanofiltrationthermocatalysisperovskitemicropollutantswater purificationwastewater |
collection |
DOAJ |
language |
English |
format |
Article |
sources |
DOAJ |
author |
Katarzyna Janowska Xianzheng Ma Vittorio Boffa Mads Koustrup Jørgensen Victor M. Candelario |
spellingShingle |
Katarzyna Janowska Xianzheng Ma Vittorio Boffa Mads Koustrup Jørgensen Victor M. Candelario Combined Nanofiltration and Thermocatalysis for the Simultaneous Degradation of Micropollutants, Fouling Mitigation and Water Purification Membranes nanofiltration thermocatalysis perovskite micropollutants water purification wastewater |
author_facet |
Katarzyna Janowska Xianzheng Ma Vittorio Boffa Mads Koustrup Jørgensen Victor M. Candelario |
author_sort |
Katarzyna Janowska |
title |
Combined Nanofiltration and Thermocatalysis for the Simultaneous Degradation of Micropollutants, Fouling Mitigation and Water Purification |
title_short |
Combined Nanofiltration and Thermocatalysis for the Simultaneous Degradation of Micropollutants, Fouling Mitigation and Water Purification |
title_full |
Combined Nanofiltration and Thermocatalysis for the Simultaneous Degradation of Micropollutants, Fouling Mitigation and Water Purification |
title_fullStr |
Combined Nanofiltration and Thermocatalysis for the Simultaneous Degradation of Micropollutants, Fouling Mitigation and Water Purification |
title_full_unstemmed |
Combined Nanofiltration and Thermocatalysis for the Simultaneous Degradation of Micropollutants, Fouling Mitigation and Water Purification |
title_sort |
combined nanofiltration and thermocatalysis for the simultaneous degradation of micropollutants, fouling mitigation and water purification |
publisher |
MDPI AG |
series |
Membranes |
issn |
2077-0375 |
publishDate |
2021-08-01 |
description |
Due to progressive limitation of access to clean drinkable water, it is nowadays a priority to find an effective method of water purification from those emerging organic contaminants, which might have potentially harmful and irreversible effects on living organisms and environment. This manuscript reports the development of a new strategy for water purification, which combines a novel and recently developed Al<sub>2</sub>O<sub>3</sub>-doped silica nanofiltration membrane with a thermocatalytic perovskite, namely cerium-doped strontium ferrate (CSF). The thermocatalytic activity of CSF offers the opportunity to degrade organic pollutants with no light and without input of chemical oxidants, providing simplicity of operation. Moreover, our studies on real samples of secondary effluent from wastewater treatment showed that the thermocatalyst has the ability to degrade also part of the non-toxic organic matter, which allows for reducing the chemical oxygen demand of the retentate and mitigating membrane fouling during filtration. Therefore, the new technology is effective in the production of clean feed and permeate and has a potential to be used in degradation of micropollutants in water treatment. |
topic |
nanofiltration thermocatalysis perovskite micropollutants water purification wastewater |
url |
https://www.mdpi.com/2077-0375/11/8/639 |
work_keys_str_mv |
AT katarzynajanowska combinednanofiltrationandthermocatalysisforthesimultaneousdegradationofmicropollutantsfoulingmitigationandwaterpurification AT xianzhengma combinednanofiltrationandthermocatalysisforthesimultaneousdegradationofmicropollutantsfoulingmitigationandwaterpurification AT vittorioboffa combinednanofiltrationandthermocatalysisforthesimultaneousdegradationofmicropollutantsfoulingmitigationandwaterpurification AT madskoustrupjørgensen combinednanofiltrationandthermocatalysisforthesimultaneousdegradationofmicropollutantsfoulingmitigationandwaterpurification AT victormcandelario combinednanofiltrationandthermocatalysisforthesimultaneousdegradationofmicropollutantsfoulingmitigationandwaterpurification |
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1721191642493353984 |