MAX-DOAS retrieval of aerosol extinction properties in Madrid, Spain

Multi-axis differential optical absorption spectroscopy (MAX-DOAS) measurements were performed in the urban environment of Madrid, Spain, from March to September 2015. The O<sub>4</sub> absorption in the ultraviolet (UV) spectral region was used to retrieve the aerosol extinction profile...

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Main Authors: S. Wang, C. A. Cuevas, U. Frieß, A. Saiz-Lopez
Format: Article
Language:English
Published: Copernicus Publications 2016-10-01
Series:Atmospheric Measurement Techniques
Online Access:http://www.atmos-meas-tech.net/9/5089/2016/amt-9-5089-2016.pdf
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spelling doaj-aa6c0f612eb14518a3daeba2477165962020-11-24T22:21:40ZengCopernicus PublicationsAtmospheric Measurement Techniques1867-13811867-85482016-10-019105089510110.5194/amt-9-5089-2016MAX-DOAS retrieval of aerosol extinction properties in Madrid, SpainS. Wang0C. A. Cuevas1U. Frieß2A. Saiz-Lopez3Department of Atmospheric Chemistry and Climate, Institute of Physical Chemistry Rocasolano, CSIC, 28006 Madrid, SpainDepartment of Atmospheric Chemistry and Climate, Institute of Physical Chemistry Rocasolano, CSIC, 28006 Madrid, SpainInstitute of Environmental Physics, University of Heidelberg, 69120 Heidelberg, GermanyDepartment of Atmospheric Chemistry and Climate, Institute of Physical Chemistry Rocasolano, CSIC, 28006 Madrid, SpainMulti-axis differential optical absorption spectroscopy (MAX-DOAS) measurements were performed in the urban environment of Madrid, Spain, from March to September 2015. The O<sub>4</sub> absorption in the ultraviolet (UV) spectral region was used to retrieve the aerosol extinction profile using an inversion algorithm. The results show a good agreement between the hourly retrieved aerosol optical depth (AOD) and the correlative Aerosol Robotic Network (AERONET) product, with a correlation coefficient of <i>R</i> =  0.87. Higher AODs are found in the summer season due to the more frequent occurrence of Saharan dust intrusions. The surface aerosol extinction coefficient as retrieved by the MAX-DOAS measurements was also compared to in situ PM<sub>2.5</sub> concentrations. The level of agreement between both measurements indicates that the MAX-DOAS retrieval has the ability to characterize the extinction of aerosol particles near the surface. The retrieval algorithm was also used to study a case of severe dust intrusion on 12 May 2015. The capability of the MAX-DOAS retrieval to recognize the dust event including an elevated particle layer is investigated along with air mass back-trajectory analysis.http://www.atmos-meas-tech.net/9/5089/2016/amt-9-5089-2016.pdf
collection DOAJ
language English
format Article
sources DOAJ
author S. Wang
C. A. Cuevas
U. Frieß
A. Saiz-Lopez
spellingShingle S. Wang
C. A. Cuevas
U. Frieß
A. Saiz-Lopez
MAX-DOAS retrieval of aerosol extinction properties in Madrid, Spain
Atmospheric Measurement Techniques
author_facet S. Wang
C. A. Cuevas
U. Frieß
A. Saiz-Lopez
author_sort S. Wang
title MAX-DOAS retrieval of aerosol extinction properties in Madrid, Spain
title_short MAX-DOAS retrieval of aerosol extinction properties in Madrid, Spain
title_full MAX-DOAS retrieval of aerosol extinction properties in Madrid, Spain
title_fullStr MAX-DOAS retrieval of aerosol extinction properties in Madrid, Spain
title_full_unstemmed MAX-DOAS retrieval of aerosol extinction properties in Madrid, Spain
title_sort max-doas retrieval of aerosol extinction properties in madrid, spain
publisher Copernicus Publications
series Atmospheric Measurement Techniques
issn 1867-1381
1867-8548
publishDate 2016-10-01
description Multi-axis differential optical absorption spectroscopy (MAX-DOAS) measurements were performed in the urban environment of Madrid, Spain, from March to September 2015. The O<sub>4</sub> absorption in the ultraviolet (UV) spectral region was used to retrieve the aerosol extinction profile using an inversion algorithm. The results show a good agreement between the hourly retrieved aerosol optical depth (AOD) and the correlative Aerosol Robotic Network (AERONET) product, with a correlation coefficient of <i>R</i> =  0.87. Higher AODs are found in the summer season due to the more frequent occurrence of Saharan dust intrusions. The surface aerosol extinction coefficient as retrieved by the MAX-DOAS measurements was also compared to in situ PM<sub>2.5</sub> concentrations. The level of agreement between both measurements indicates that the MAX-DOAS retrieval has the ability to characterize the extinction of aerosol particles near the surface. The retrieval algorithm was also used to study a case of severe dust intrusion on 12 May 2015. The capability of the MAX-DOAS retrieval to recognize the dust event including an elevated particle layer is investigated along with air mass back-trajectory analysis.
url http://www.atmos-meas-tech.net/9/5089/2016/amt-9-5089-2016.pdf
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