Magnetic resonance probing of ground state in the mixed valence correlated topological insulator SmB6

Abstract Introducing of topological insulator concept for fluctuating valence compound – samarium hexaboride – has recently initiated a new round of studies aimed to clarify the nature of the ground state in this extraordinary system with strong electron correlations. Here we discuss the data of mag...

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Main Authors: S. V. Demishev, M. I. Gilmanov, A. N. Samarin, A. V. Semeno, N. E. Sluchanko, N. A. Samarin, A. V. Bogach, N. Yu. Shitsevalova, V. B. Filipov, M. S. Karasev, V. V. Glushkov
Format: Article
Language:English
Published: Nature Publishing Group 2018-05-01
Series:Scientific Reports
Online Access:https://doi.org/10.1038/s41598-018-25464-y
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spelling doaj-b26175ead1d5402d838c360c694fc6392020-12-08T04:40:41ZengNature Publishing GroupScientific Reports2045-23222018-05-01811810.1038/s41598-018-25464-yMagnetic resonance probing of ground state in the mixed valence correlated topological insulator SmB6S. V. Demishev0M. I. Gilmanov1A. N. Samarin2A. V. Semeno3N. E. Sluchanko4N. A. Samarin5A. V. Bogach6N. Yu. Shitsevalova7V. B. Filipov8M. S. Karasev9V. V. Glushkov10Moscow Institute of Physics and Technology, DolgoprudnyMoscow Institute of Physics and Technology, DolgoprudnyProkhorov General Physics Institute of the Russian Academy of SciencesMoscow Institute of Physics and Technology, DolgoprudnyMoscow Institute of Physics and Technology, DolgoprudnyProkhorov General Physics Institute of the Russian Academy of SciencesProkhorov General Physics Institute of the Russian Academy of SciencesInstitute for Problems of Materials Science of NASUInstitute for Problems of Materials Science of NASUProkhorov General Physics Institute of the Russian Academy of SciencesMoscow Institute of Physics and Technology, DolgoprudnyAbstract Introducing of topological insulator concept for fluctuating valence compound – samarium hexaboride – has recently initiated a new round of studies aimed to clarify the nature of the ground state in this extraordinary system with strong electron correlations. Here we discuss the data of magnetic resonance in the pristine single crystals of SmB6 measured in 60 GHz cavity experiments at temperatures 1.8–300 K. The microwave study as well as the DC resistivity and Hall effect measurements performed for the different states of SmB6 [110] surface prove definitely the existence of the layer with metallic conductivity increasing under lowering temperature below 5 K. Four lines with the g-factors g ≈ 2 are found to contribute to the ESR-like absorption spectrum that may be attributed to intrinsic paramagnetic centers on the sample’s surface, which are robust with respect to the surface treatment. The temperature dependence of integrated intensity I(T) for main paramagnetic signal is found to demonstrate anomalous critical behavior I(T) ~ (T * − T)ν with characteristic temperature T *  = 5.34 ± 0.05 K and exponent ν = 0.38 ± 0.03 indicating possible magnetic transition at the SmB6 [110] surface. Additional resonant magnetoabsorption line, which may be associated with either donor-like defects or cyclotron resonance mode corresponding to the mass m c  ~ 1.2m 0, is reported.https://doi.org/10.1038/s41598-018-25464-y
collection DOAJ
language English
format Article
sources DOAJ
author S. V. Demishev
M. I. Gilmanov
A. N. Samarin
A. V. Semeno
N. E. Sluchanko
N. A. Samarin
A. V. Bogach
N. Yu. Shitsevalova
V. B. Filipov
M. S. Karasev
V. V. Glushkov
spellingShingle S. V. Demishev
M. I. Gilmanov
A. N. Samarin
A. V. Semeno
N. E. Sluchanko
N. A. Samarin
A. V. Bogach
N. Yu. Shitsevalova
V. B. Filipov
M. S. Karasev
V. V. Glushkov
Magnetic resonance probing of ground state in the mixed valence correlated topological insulator SmB6
Scientific Reports
author_facet S. V. Demishev
M. I. Gilmanov
A. N. Samarin
A. V. Semeno
N. E. Sluchanko
N. A. Samarin
A. V. Bogach
N. Yu. Shitsevalova
V. B. Filipov
M. S. Karasev
V. V. Glushkov
author_sort S. V. Demishev
title Magnetic resonance probing of ground state in the mixed valence correlated topological insulator SmB6
title_short Magnetic resonance probing of ground state in the mixed valence correlated topological insulator SmB6
title_full Magnetic resonance probing of ground state in the mixed valence correlated topological insulator SmB6
title_fullStr Magnetic resonance probing of ground state in the mixed valence correlated topological insulator SmB6
title_full_unstemmed Magnetic resonance probing of ground state in the mixed valence correlated topological insulator SmB6
title_sort magnetic resonance probing of ground state in the mixed valence correlated topological insulator smb6
publisher Nature Publishing Group
series Scientific Reports
issn 2045-2322
publishDate 2018-05-01
description Abstract Introducing of topological insulator concept for fluctuating valence compound – samarium hexaboride – has recently initiated a new round of studies aimed to clarify the nature of the ground state in this extraordinary system with strong electron correlations. Here we discuss the data of magnetic resonance in the pristine single crystals of SmB6 measured in 60 GHz cavity experiments at temperatures 1.8–300 K. The microwave study as well as the DC resistivity and Hall effect measurements performed for the different states of SmB6 [110] surface prove definitely the existence of the layer with metallic conductivity increasing under lowering temperature below 5 K. Four lines with the g-factors g ≈ 2 are found to contribute to the ESR-like absorption spectrum that may be attributed to intrinsic paramagnetic centers on the sample’s surface, which are robust with respect to the surface treatment. The temperature dependence of integrated intensity I(T) for main paramagnetic signal is found to demonstrate anomalous critical behavior I(T) ~ (T * − T)ν with characteristic temperature T *  = 5.34 ± 0.05 K and exponent ν = 0.38 ± 0.03 indicating possible magnetic transition at the SmB6 [110] surface. Additional resonant magnetoabsorption line, which may be associated with either donor-like defects or cyclotron resonance mode corresponding to the mass m c  ~ 1.2m 0, is reported.
url https://doi.org/10.1038/s41598-018-25464-y
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