Tracking the coherent generation of polaron pairs in conjugated polymers

Tracking the coherent generation of polaron pairs in conjugated polymers

Understanding of charge transfer dynamics is essential to the design of high-performance organic semiconductors for optoelectronic applications. Here, the authors show that excitons, polaron pairs and a long-lived vibrational mode are strongly coupled to each other up to 1 picosecond in polythiophen...

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Main Authors: Antonietta De Sio, Filippo Troiani, Margherita Maiuri, Julien Réhault, Ephraim Sommer, James Lim, Susana F. Huelga, Martin B. Plenio, Carlo Andrea Rozzi, Giulio Cerullo, Elisa Molinari, Christoph Lienau
Format: Article
Language:English
Published: Nature Publishing Group 2016-12-01
Series:Nature Communications
Online Access:https://doi.org/10.1038/ncomms13742
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spelling doaj-c510d6331ebf423594e100feadc4b1752021-05-11T10:49:55ZengNature Publishing GroupNature Communications2041-17232016-12-01711810.1038/ncomms13742Tracking the coherent generation of polaron pairs in conjugated polymersAntonietta De Sio0Filippo Troiani1Margherita Maiuri2Julien Réhault3Ephraim Sommer4James Lim5Susana F. Huelga6Martin B. Plenio7Carlo Andrea Rozzi8Giulio Cerullo9Elisa Molinari10Christoph Lienau11Institut für Physik, Carl von Ossietzky UniversitätIstituto Nanoscienze—CNRDipartimento di Fisica, IFN-CNR, Politecnico di MilanoDipartimento di Fisica, IFN-CNR, Politecnico di MilanoInstitut für Physik, Carl von Ossietzky UniversitätInstitut für Theoretische Physik and IQST, Universität UlmInstitut für Theoretische Physik and IQST, Universität UlmInstitut für Theoretische Physik and IQST, Universität UlmIstituto Nanoscienze—CNRDipartimento di Fisica, IFN-CNR, Politecnico di MilanoIstituto Nanoscienze—CNRInstitut für Physik, Carl von Ossietzky UniversitätUnderstanding of charge transfer dynamics is essential to the design of high-performance organic semiconductors for optoelectronic applications. Here, the authors show that excitons, polaron pairs and a long-lived vibrational mode are strongly coupled to each other up to 1 picosecond in polythiophene.https://doi.org/10.1038/ncomms13742
collection DOAJ
language English
format Article
sources DOAJ
author Antonietta De Sio
Filippo Troiani
Margherita Maiuri
Julien Réhault
Ephraim Sommer
James Lim
Susana F. Huelga
Martin B. Plenio
Carlo Andrea Rozzi
Giulio Cerullo
Elisa Molinari
Christoph Lienau
spellingShingle Antonietta De Sio
Filippo Troiani
Margherita Maiuri
Julien Réhault
Ephraim Sommer
James Lim
Susana F. Huelga
Martin B. Plenio
Carlo Andrea Rozzi
Giulio Cerullo
Elisa Molinari
Christoph Lienau
Tracking the coherent generation of polaron pairs in conjugated polymers
Nature Communications
author_facet Antonietta De Sio
Filippo Troiani
Margherita Maiuri
Julien Réhault
Ephraim Sommer
James Lim
Susana F. Huelga
Martin B. Plenio
Carlo Andrea Rozzi
Giulio Cerullo
Elisa Molinari
Christoph Lienau
author_sort Antonietta De Sio
title Tracking the coherent generation of polaron pairs in conjugated polymers
title_short Tracking the coherent generation of polaron pairs in conjugated polymers
title_full Tracking the coherent generation of polaron pairs in conjugated polymers
title_fullStr Tracking the coherent generation of polaron pairs in conjugated polymers
title_full_unstemmed Tracking the coherent generation of polaron pairs in conjugated polymers
title_sort tracking the coherent generation of polaron pairs in conjugated polymers
publisher Nature Publishing Group
series Nature Communications
issn 2041-1723
publishDate 2016-12-01
description Understanding of charge transfer dynamics is essential to the design of high-performance organic semiconductors for optoelectronic applications. Here, the authors show that excitons, polaron pairs and a long-lived vibrational mode are strongly coupled to each other up to 1 picosecond in polythiophene.
url https://doi.org/10.1038/ncomms13742
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