Graphene Oxide/Polystyrene Bilayer Gate Dielectrics for Low-Voltage Organic Field-Effect Transistors

Here, we report on the use of a graphene oxide (GO)/polystyrene (PS) bilayer as a gate dielectric for low-voltage organic field-effect transistors (OFETs). The hydrophilic functional groups of GO cause surface trapping and high gate leakage, which can be overcome by introducing a layer of PS&#82...

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Main Authors: Sooji Nam, Yong Jin Jeong, Joo Yeon Kim, Hansol Yang, Jaeyoung Jang
Format: Article
Language:English
Published: MDPI AG 2018-12-01
Series:Applied Sciences
Subjects:
Online Access:https://www.mdpi.com/2076-3417/9/1/2
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spelling doaj-cae796c2c7a64e5085801d7ef52677a62020-11-24T22:05:03ZengMDPI AGApplied Sciences2076-34172018-12-0191210.3390/app9010002app9010002Graphene Oxide/Polystyrene Bilayer Gate Dielectrics for Low-Voltage Organic Field-Effect TransistorsSooji Nam0Yong Jin Jeong1Joo Yeon Kim2Hansol Yang3Jaeyoung Jang4Realistic Display Research Group, Electronics and Telecommunications Research Institute, Daejeon 34129, KoreaDepartment of Energy Engineering, Hanyang University, Seoul 04763, KoreaRealistic Display Research Group, Electronics and Telecommunications Research Institute, Daejeon 34129, KoreaDepartment of Energy Engineering, Hanyang University, Seoul 04763, KoreaDepartment of Energy Engineering, Hanyang University, Seoul 04763, KoreaHere, we report on the use of a graphene oxide (GO)/polystyrene (PS) bilayer as a gate dielectric for low-voltage organic field-effect transistors (OFETs). The hydrophilic functional groups of GO cause surface trapping and high gate leakage, which can be overcome by introducing a layer of PS&#8212;a hydrophobic polymer&#8212;onto the top surface of GO. The GO/PS gate dielectric shows reduced surface roughness and gate leakage while maintaining a high capacitance of 37.8 nF cm<sup>&#8722;2</sup>. The resulting OFETs show high-performance operation with a high mobility of 1.05 cm<sup>2</sup> V<sup>&#8722;1</sup> s<sup>&#8722;1</sup> within a low operating voltage of &#8722;5 V.https://www.mdpi.com/2076-3417/9/1/2graphene oxidepolystyrenegate dielectriclow voltageorganic field-effect transistor
collection DOAJ
language English
format Article
sources DOAJ
author Sooji Nam
Yong Jin Jeong
Joo Yeon Kim
Hansol Yang
Jaeyoung Jang
spellingShingle Sooji Nam
Yong Jin Jeong
Joo Yeon Kim
Hansol Yang
Jaeyoung Jang
Graphene Oxide/Polystyrene Bilayer Gate Dielectrics for Low-Voltage Organic Field-Effect Transistors
Applied Sciences
graphene oxide
polystyrene
gate dielectric
low voltage
organic field-effect transistor
author_facet Sooji Nam
Yong Jin Jeong
Joo Yeon Kim
Hansol Yang
Jaeyoung Jang
author_sort Sooji Nam
title Graphene Oxide/Polystyrene Bilayer Gate Dielectrics for Low-Voltage Organic Field-Effect Transistors
title_short Graphene Oxide/Polystyrene Bilayer Gate Dielectrics for Low-Voltage Organic Field-Effect Transistors
title_full Graphene Oxide/Polystyrene Bilayer Gate Dielectrics for Low-Voltage Organic Field-Effect Transistors
title_fullStr Graphene Oxide/Polystyrene Bilayer Gate Dielectrics for Low-Voltage Organic Field-Effect Transistors
title_full_unstemmed Graphene Oxide/Polystyrene Bilayer Gate Dielectrics for Low-Voltage Organic Field-Effect Transistors
title_sort graphene oxide/polystyrene bilayer gate dielectrics for low-voltage organic field-effect transistors
publisher MDPI AG
series Applied Sciences
issn 2076-3417
publishDate 2018-12-01
description Here, we report on the use of a graphene oxide (GO)/polystyrene (PS) bilayer as a gate dielectric for low-voltage organic field-effect transistors (OFETs). The hydrophilic functional groups of GO cause surface trapping and high gate leakage, which can be overcome by introducing a layer of PS&#8212;a hydrophobic polymer&#8212;onto the top surface of GO. The GO/PS gate dielectric shows reduced surface roughness and gate leakage while maintaining a high capacitance of 37.8 nF cm<sup>&#8722;2</sup>. The resulting OFETs show high-performance operation with a high mobility of 1.05 cm<sup>2</sup> V<sup>&#8722;1</sup> s<sup>&#8722;1</sup> within a low operating voltage of &#8722;5 V.
topic graphene oxide
polystyrene
gate dielectric
low voltage
organic field-effect transistor
url https://www.mdpi.com/2076-3417/9/1/2
work_keys_str_mv AT soojinam grapheneoxidepolystyrenebilayergatedielectricsforlowvoltageorganicfieldeffecttransistors
AT yongjinjeong grapheneoxidepolystyrenebilayergatedielectricsforlowvoltageorganicfieldeffecttransistors
AT jooyeonkim grapheneoxidepolystyrenebilayergatedielectricsforlowvoltageorganicfieldeffecttransistors
AT hansolyang grapheneoxidepolystyrenebilayergatedielectricsforlowvoltageorganicfieldeffecttransistors
AT jaeyoungjang grapheneoxidepolystyrenebilayergatedielectricsforlowvoltageorganicfieldeffecttransistors
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