High-Performance Flexible Supercapacitors obtained via Recycled Jute: Bio-Waste to Energy Storage Approach

Abstract In search of affordable, flexible, lightweight, efficient and stable supercapacitors, metal oxides have been shown to provide high charge storage capacity but with poor cyclic stability due to structural damage occurring during the redox process. Here, we develop an efficient flexible super...

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Main Authors: Camila Zequine, C. K. Ranaweera, Z. Wang, Petar R. Dvornic, P. K. Kahol, Sweta Singh, Prashant Tripathi, O. N. Srivastava, Satbir Singh, Bipin Kumar Gupta, Gautam Gupta, Ram K. Gupta
Format: Article
Language:English
Published: Nature Publishing Group 2017-04-01
Series:Scientific Reports
Online Access:https://doi.org/10.1038/s41598-017-01319-w
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spelling doaj-d868c6b6616a4957b319798d0059d8262020-12-08T01:50:28ZengNature Publishing GroupScientific Reports2045-23222017-04-017111210.1038/s41598-017-01319-wHigh-Performance Flexible Supercapacitors obtained via Recycled Jute: Bio-Waste to Energy Storage ApproachCamila Zequine0C. K. Ranaweera1Z. Wang2Petar R. Dvornic3P. K. Kahol4Sweta Singh5Prashant Tripathi6O. N. Srivastava7Satbir Singh8Bipin Kumar Gupta9Gautam Gupta10Ram K. Gupta11Department of Chemistry, Pittsburg State UniversityDepartment of Chemistry, Pittsburg State UniversityDepartment of Chemistry, Pittsburg State UniversityDepartment of Chemistry, Pittsburg State UniversityDepartment of Physics, Pittsburg State UniversityDepartment of Physics, Banaras Hindu UniversityDepartment of Physics, Banaras Hindu UniversityDepartment of Physics, Banaras Hindu UniversityCSIR -National Physical LaboratoryCSIR -National Physical LaboratoryMaterials Physics and Applications (MPA-11), Los Alamos National LaboratoryDepartment of Chemistry, Pittsburg State UniversityAbstract In search of affordable, flexible, lightweight, efficient and stable supercapacitors, metal oxides have been shown to provide high charge storage capacity but with poor cyclic stability due to structural damage occurring during the redox process. Here, we develop an efficient flexible supercapacitor obtained by carbonizing abundantly available and recyclable jute. The active material was synthesized from jute by a facile hydrothermal method and its electrochemical performance was further enhanced by chemical activation. Specific capacitance of 408 F/g at 1 mV/s using CV and 185 F/g at 500 mA/g using charge-discharge measurements with excellent flexibility (~100% retention in charge storage capacity on bending) were observed. The cyclic stability test confirmed no loss in the charge storage capacity of the electrode even after 5,000 charge-discharge measurements. In addition, a supercapacitor device fabricated using this carbonized jute showed promising specific capacitance of about 51 F/g, and improvement of over 60% in the charge storage capacity on increasing temperature from 5 to 75 °C. Based on these results, we propose that recycled jute should be considered for fabrication of high-performance flexible energy storage devices at extremely low cost.https://doi.org/10.1038/s41598-017-01319-w
collection DOAJ
language English
format Article
sources DOAJ
author Camila Zequine
C. K. Ranaweera
Z. Wang
Petar R. Dvornic
P. K. Kahol
Sweta Singh
Prashant Tripathi
O. N. Srivastava
Satbir Singh
Bipin Kumar Gupta
Gautam Gupta
Ram K. Gupta
spellingShingle Camila Zequine
C. K. Ranaweera
Z. Wang
Petar R. Dvornic
P. K. Kahol
Sweta Singh
Prashant Tripathi
O. N. Srivastava
Satbir Singh
Bipin Kumar Gupta
Gautam Gupta
Ram K. Gupta
High-Performance Flexible Supercapacitors obtained via Recycled Jute: Bio-Waste to Energy Storage Approach
Scientific Reports
author_facet Camila Zequine
C. K. Ranaweera
Z. Wang
Petar R. Dvornic
P. K. Kahol
Sweta Singh
Prashant Tripathi
O. N. Srivastava
Satbir Singh
Bipin Kumar Gupta
Gautam Gupta
Ram K. Gupta
author_sort Camila Zequine
title High-Performance Flexible Supercapacitors obtained via Recycled Jute: Bio-Waste to Energy Storage Approach
title_short High-Performance Flexible Supercapacitors obtained via Recycled Jute: Bio-Waste to Energy Storage Approach
title_full High-Performance Flexible Supercapacitors obtained via Recycled Jute: Bio-Waste to Energy Storage Approach
title_fullStr High-Performance Flexible Supercapacitors obtained via Recycled Jute: Bio-Waste to Energy Storage Approach
title_full_unstemmed High-Performance Flexible Supercapacitors obtained via Recycled Jute: Bio-Waste to Energy Storage Approach
title_sort high-performance flexible supercapacitors obtained via recycled jute: bio-waste to energy storage approach
publisher Nature Publishing Group
series Scientific Reports
issn 2045-2322
publishDate 2017-04-01
description Abstract In search of affordable, flexible, lightweight, efficient and stable supercapacitors, metal oxides have been shown to provide high charge storage capacity but with poor cyclic stability due to structural damage occurring during the redox process. Here, we develop an efficient flexible supercapacitor obtained by carbonizing abundantly available and recyclable jute. The active material was synthesized from jute by a facile hydrothermal method and its electrochemical performance was further enhanced by chemical activation. Specific capacitance of 408 F/g at 1 mV/s using CV and 185 F/g at 500 mA/g using charge-discharge measurements with excellent flexibility (~100% retention in charge storage capacity on bending) were observed. The cyclic stability test confirmed no loss in the charge storage capacity of the electrode even after 5,000 charge-discharge measurements. In addition, a supercapacitor device fabricated using this carbonized jute showed promising specific capacitance of about 51 F/g, and improvement of over 60% in the charge storage capacity on increasing temperature from 5 to 75 °C. Based on these results, we propose that recycled jute should be considered for fabrication of high-performance flexible energy storage devices at extremely low cost.
url https://doi.org/10.1038/s41598-017-01319-w
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