Interplay between electrochemical reactions and mechanical responses in silicon–graphite anodes and its impact on degradation

The degradation in silicon-graphite anodes is originated from Li ion crosstalk between silicon and graphite, and the pressure-induced staging transition of the graphite. Here, the authors demonstrate a prismatic cell with improved volumetric energy density and cycle stability by targeted solving abo...

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Main Authors: Junhyuk Moon, Heung Chan Lee, Heechul Jung, Shinya Wakita, Sungnim Cho, Jaegu Yoon, Joowook Lee, Atsushi Ueda, Bokkyu Choi, Sihyung Lee, Kimihiko Ito, Yoshimi Kubo, Alan Christian Lim, Jeong Gil Seo, Jungho Yoo, Seungyeon Lee, Yongnam Ham, Woonjoong Baek, Young-Gyoon Ryu, In Taek Han
Format: Article
Language:English
Published: Nature Publishing Group 2021-05-01
Series:Nature Communications
Online Access:https://doi.org/10.1038/s41467-021-22662-7
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spelling doaj-f9e391c6fc6e418d86cbd848b66becad2021-05-11T14:49:58ZengNature Publishing GroupNature Communications2041-17232021-05-0112111010.1038/s41467-021-22662-7Interplay between electrochemical reactions and mechanical responses in silicon–graphite anodes and its impact on degradationJunhyuk Moon0Heung Chan Lee1Heechul Jung2Shinya Wakita3Sungnim Cho4Jaegu Yoon5Joowook Lee6Atsushi Ueda7Bokkyu Choi8Sihyung Lee9Kimihiko Ito10Yoshimi Kubo11Alan Christian Lim12Jeong Gil Seo13Jungho Yoo14Seungyeon Lee15Yongnam Ham16Woonjoong Baek17Young-Gyoon Ryu18In Taek Han19Samsung Advanced Institute of TechnologySamsung Advanced Institute of TechnologySamsung Advanced Institute of TechnologySamsung Advanced Institute of TechnologySamsung Advanced Institute of TechnologySamsung Advanced Institute of TechnologySamsung Advanced Institute of TechnologySamsung Advanced Institute of TechnologySamsung Advanced Institute of TechnologySamsung Advanced Institute of TechnologyC4GR-GREEN, National Institute for Materials ScienceC4GR-GREEN, National Institute for Materials ScienceDepartment of Chemical Engineering, Hanyang UniversityDepartment of Chemical Engineering, Hanyang UniversityNational NanoFab CenterSamsung Advanced Institute of TechnologySamsung Advanced Institute of TechnologySamsung Advanced Institute of TechnologySamsung Advanced Institute of TechnologySamsung Advanced Institute of TechnologyThe degradation in silicon-graphite anodes is originated from Li ion crosstalk between silicon and graphite, and the pressure-induced staging transition of the graphite. Here, the authors demonstrate a prismatic cell with improved volumetric energy density and cycle stability by targeted solving above issues.https://doi.org/10.1038/s41467-021-22662-7
collection DOAJ
language English
format Article
sources DOAJ
author Junhyuk Moon
Heung Chan Lee
Heechul Jung
Shinya Wakita
Sungnim Cho
Jaegu Yoon
Joowook Lee
Atsushi Ueda
Bokkyu Choi
Sihyung Lee
Kimihiko Ito
Yoshimi Kubo
Alan Christian Lim
Jeong Gil Seo
Jungho Yoo
Seungyeon Lee
Yongnam Ham
Woonjoong Baek
Young-Gyoon Ryu
In Taek Han
spellingShingle Junhyuk Moon
Heung Chan Lee
Heechul Jung
Shinya Wakita
Sungnim Cho
Jaegu Yoon
Joowook Lee
Atsushi Ueda
Bokkyu Choi
Sihyung Lee
Kimihiko Ito
Yoshimi Kubo
Alan Christian Lim
Jeong Gil Seo
Jungho Yoo
Seungyeon Lee
Yongnam Ham
Woonjoong Baek
Young-Gyoon Ryu
In Taek Han
Interplay between electrochemical reactions and mechanical responses in silicon–graphite anodes and its impact on degradation
Nature Communications
author_facet Junhyuk Moon
Heung Chan Lee
Heechul Jung
Shinya Wakita
Sungnim Cho
Jaegu Yoon
Joowook Lee
Atsushi Ueda
Bokkyu Choi
Sihyung Lee
Kimihiko Ito
Yoshimi Kubo
Alan Christian Lim
Jeong Gil Seo
Jungho Yoo
Seungyeon Lee
Yongnam Ham
Woonjoong Baek
Young-Gyoon Ryu
In Taek Han
author_sort Junhyuk Moon
title Interplay between electrochemical reactions and mechanical responses in silicon–graphite anodes and its impact on degradation
title_short Interplay between electrochemical reactions and mechanical responses in silicon–graphite anodes and its impact on degradation
title_full Interplay between electrochemical reactions and mechanical responses in silicon–graphite anodes and its impact on degradation
title_fullStr Interplay between electrochemical reactions and mechanical responses in silicon–graphite anodes and its impact on degradation
title_full_unstemmed Interplay between electrochemical reactions and mechanical responses in silicon–graphite anodes and its impact on degradation
title_sort interplay between electrochemical reactions and mechanical responses in silicon–graphite anodes and its impact on degradation
publisher Nature Publishing Group
series Nature Communications
issn 2041-1723
publishDate 2021-05-01
description The degradation in silicon-graphite anodes is originated from Li ion crosstalk between silicon and graphite, and the pressure-induced staging transition of the graphite. Here, the authors demonstrate a prismatic cell with improved volumetric energy density and cycle stability by targeted solving above issues.
url https://doi.org/10.1038/s41467-021-22662-7
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