Nonlinear Ultrafast Excitation and Two-Dimensional Terahertz Spectroscopy of Solids
Ultrafast spectroscopy allows us to probe and understand material properties. With it, we can measure phonon-polaritons (optical phonons coupled with light) and the resulting dispersion curve in lithium niobate. Customizing the excitation source in ultrafast measurements can excite phonon modes to l...
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ndltd-BGMYU2-oai-scholarsarchive.byu.edu-etd-101992021-09-22T05:00:51Z Nonlinear Ultrafast Excitation and Two-Dimensional Terahertz Spectroscopy of Solids Knighton, Brittany E. Ultrafast spectroscopy allows us to probe and understand material properties. With it, we can measure phonon-polaritons (optical phonons coupled with light) and the resulting dispersion curve in lithium niobate. Customizing the excitation source in ultrafast measurements can excite phonon modes to large amplitudes, allowing the experimental exploration of the Potential Energy Surface in solids. However, stronger pump fluences and bigger signal isn't always the answer in ultrafast spectroscopy. When sample signals and their nonlinear and mechanisms cannot be distinguished with 1D measurements, simple 2D THz measurements are a great place to start searching for distinct factors as was the case in cadmium tungstate. 2D measurements when paired with modeling and first principles calculations can reveal cutting edge information about exciting materials. 2021-07-27T07:00:00Z text application/pdf https://scholarsarchive.byu.edu/etd/9190 https://scholarsarchive.byu.edu/cgi/viewcontent.cgi?article=10199&context=etd https://lib.byu.edu/about/copyright/ Theses and Dissertations BYU ScholarsArchive ultrafast spectroscopy nonlinear phononics trilinear coupling terahertz ultrafast 2D terahertz spectroscopy Physical Sciences and Mathematics |
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ultrafast spectroscopy nonlinear phononics trilinear coupling terahertz ultrafast 2D terahertz spectroscopy Physical Sciences and Mathematics |
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ultrafast spectroscopy nonlinear phononics trilinear coupling terahertz ultrafast 2D terahertz spectroscopy Physical Sciences and Mathematics Knighton, Brittany E. Nonlinear Ultrafast Excitation and Two-Dimensional Terahertz Spectroscopy of Solids |
description |
Ultrafast spectroscopy allows us to probe and understand material properties. With it, we can measure phonon-polaritons (optical phonons coupled with light) and the resulting dispersion curve in lithium niobate. Customizing the excitation source in ultrafast measurements can excite phonon modes to large amplitudes, allowing the experimental exploration of the Potential Energy Surface in solids. However, stronger pump fluences and bigger signal isn't always the answer in ultrafast spectroscopy. When sample signals and their nonlinear and mechanisms cannot be distinguished with 1D measurements, simple 2D THz measurements are a great place to start searching for distinct factors as was the case in cadmium tungstate. 2D measurements when paired with modeling and first principles calculations can reveal cutting edge information about exciting materials. |
author |
Knighton, Brittany E. |
author_facet |
Knighton, Brittany E. |
author_sort |
Knighton, Brittany E. |
title |
Nonlinear Ultrafast Excitation and Two-Dimensional Terahertz Spectroscopy of Solids |
title_short |
Nonlinear Ultrafast Excitation and Two-Dimensional Terahertz Spectroscopy of Solids |
title_full |
Nonlinear Ultrafast Excitation and Two-Dimensional Terahertz Spectroscopy of Solids |
title_fullStr |
Nonlinear Ultrafast Excitation and Two-Dimensional Terahertz Spectroscopy of Solids |
title_full_unstemmed |
Nonlinear Ultrafast Excitation and Two-Dimensional Terahertz Spectroscopy of Solids |
title_sort |
nonlinear ultrafast excitation and two-dimensional terahertz spectroscopy of solids |
publisher |
BYU ScholarsArchive |
publishDate |
2021 |
url |
https://scholarsarchive.byu.edu/etd/9190 https://scholarsarchive.byu.edu/cgi/viewcontent.cgi?article=10199&context=etd |
work_keys_str_mv |
AT knightonbrittanye nonlinearultrafastexcitationandtwodimensionalterahertzspectroscopyofsolids |
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1719482732929613824 |