Nanoplasmonic Sensing using Metal Nanoparticles
In our modern society, we are surrounded by numerous sensors, constantly feeding us information about our physical environment. From small, wearable sensors that monitor our physiological status to large satellites orbiting around the earth, detecting global changes. Although, the performance of the...
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Linköpings universitet, Molekylär fysik
2014
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ndltd-UPSALLA1-oai-DiVA.org-liu-1118412017-01-12T05:12:58ZNanoplasmonic Sensing using Metal NanoparticlesengMartinsson, ErikLinköpings universitet, Molekylär fysikLinköpings universitet, Tekniska högskolanLinköping2014Nanoparticlessensingbiosensorsrefractive index sensingplasmonicsnanoplasmonicsIn our modern society, we are surrounded by numerous sensors, constantly feeding us information about our physical environment. From small, wearable sensors that monitor our physiological status to large satellites orbiting around the earth, detecting global changes. Although, the performance of these sensors have been significantly improved during the last decades there is still a demand for faster and more reliable sensing systems with improved sensitivity and selectivity. The rapid progress in nanofabrication techniques has made a profound impact for the development of small, novel sensors that enables miniaturization and integration. A specific area where nanostructures are especially attractive is biochemical sensing, where the exceptional properties of nanomaterials can be utilized in order to detect and analyze biomolecular interactions. The focus of this thesis is to investigate plasmonic nanoparticles composed of gold or silver and optimize their performance as signal transducers in optical biosensors. Metal nanoparticles exhibit unique optical properties due to excitation of localized surface plasmons, which makes them highly sensitive probes for detecting small, local changes in their surrounding environment, for instance the binding of a biomolecule to the nanoparticle surface. This is the basic principle behind nanoplasmonic sensing based on refractometric detection, a sensing scheme that offers real-time and label-free detection of molecular interactions. This thesis shows that the sensitivity for detecting local refractive index changes is highly dependent on the geometry of the metal nanoparticles, their interaction with neighboring particles and their chemical composition and functionalization. An increased knowledge about how these parameters affects the sensitivity is essential when developing nanoplasmonic sensing devices with high performance based on metal nanoparticles. Doctoral thesis, comprehensive summaryinfo:eu-repo/semantics/doctoralThesistexthttp://urn.kb.se/resolve?urn=urn:nbn:se:liu:diva-111841urn:isbn:978-91-7519-223-9 (print)doi:10.3384/diss.diva-111841Linköping Studies in Science and Technology. Dissertations, 0345-7524 ; 1624application/pdfinfo:eu-repo/semantics/openAccess |
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language |
English |
format |
Doctoral Thesis |
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topic |
Nanoparticles sensing biosensors refractive index sensing plasmonics nanoplasmonics |
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Nanoparticles sensing biosensors refractive index sensing plasmonics nanoplasmonics Martinsson, Erik Nanoplasmonic Sensing using Metal Nanoparticles |
description |
In our modern society, we are surrounded by numerous sensors, constantly feeding us information about our physical environment. From small, wearable sensors that monitor our physiological status to large satellites orbiting around the earth, detecting global changes. Although, the performance of these sensors have been significantly improved during the last decades there is still a demand for faster and more reliable sensing systems with improved sensitivity and selectivity. The rapid progress in nanofabrication techniques has made a profound impact for the development of small, novel sensors that enables miniaturization and integration. A specific area where nanostructures are especially attractive is biochemical sensing, where the exceptional properties of nanomaterials can be utilized in order to detect and analyze biomolecular interactions. The focus of this thesis is to investigate plasmonic nanoparticles composed of gold or silver and optimize their performance as signal transducers in optical biosensors. Metal nanoparticles exhibit unique optical properties due to excitation of localized surface plasmons, which makes them highly sensitive probes for detecting small, local changes in their surrounding environment, for instance the binding of a biomolecule to the nanoparticle surface. This is the basic principle behind nanoplasmonic sensing based on refractometric detection, a sensing scheme that offers real-time and label-free detection of molecular interactions. This thesis shows that the sensitivity for detecting local refractive index changes is highly dependent on the geometry of the metal nanoparticles, their interaction with neighboring particles and their chemical composition and functionalization. An increased knowledge about how these parameters affects the sensitivity is essential when developing nanoplasmonic sensing devices with high performance based on metal nanoparticles. |
author |
Martinsson, Erik |
author_facet |
Martinsson, Erik |
author_sort |
Martinsson, Erik |
title |
Nanoplasmonic Sensing using Metal Nanoparticles |
title_short |
Nanoplasmonic Sensing using Metal Nanoparticles |
title_full |
Nanoplasmonic Sensing using Metal Nanoparticles |
title_fullStr |
Nanoplasmonic Sensing using Metal Nanoparticles |
title_full_unstemmed |
Nanoplasmonic Sensing using Metal Nanoparticles |
title_sort |
nanoplasmonic sensing using metal nanoparticles |
publisher |
Linköpings universitet, Molekylär fysik |
publishDate |
2014 |
url |
http://urn.kb.se/resolve?urn=urn:nbn:se:liu:diva-111841 http://nbn-resolving.de/urn:isbn:978-91-7519-223-9 (print) |
work_keys_str_mv |
AT martinssonerik nanoplasmonicsensingusingmetalnanoparticles |
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1718407750266912768 |