| Summary: | Glass microfibre waveguides offer an intriguing platform for the investigation of nonlinear effects, due to their high effective nonlinearity which arises from the tight modal confinement down to dimensions comparable to the wavelength of guided light. This thesis presents theoretical and experimental work towards achieving efficient third and second harmonic generation in silica microfibres, as well as in microfibre loop resonators for enhancing the conversion. Since microfibre resonators themselves exhibit interesting nonlinear behaviour, the polarisation dependent properties of microcoil resonators were also studied. Efficient third harmonic generation is possible through intermodal phase matching, and experiments using short tapers have demonstrated significant efficiencies up to 10
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