Thermal transport in silver-coated polymer sphere composites by the bidirectional 3 ω method

The bidirectional 3 ω method is an electrothermal technique that is commonly used to obtain the thermal conductivity of materials such as liquids, biological samples, and pastes. In this work, an epoxy-based adhesive was filled with monodisperse 10 μm polymethyl methacrylate spheres coated with silv...

Full description

Bibliographic Details
Main Authors: Chávez-Ángel, E. (Author), He, J. (Author), Kristiansen, H. (Author), Sandell, S. (Author), Wang, T. (Author), Zhang, Z. (Author)
Format: Article
Language:English
Published: American Institute of Physics Inc. 2022
Subjects:
Online Access:View Fulltext in Publisher
Description
Summary:The bidirectional 3 ω method is an electrothermal technique that is commonly used to obtain the thermal conductivity of materials such as liquids, biological samples, and pastes. In this work, an epoxy-based adhesive was filled with monodisperse 10 μm polymethyl methacrylate spheres coated with silver thin films (AgPS), such that a metallic network that dominated the thermal transport was formed through the composite. The bidirectional 3 ω method was used to obtain the thermal conductivity of the conductive adhesive at different volume fractions of AgPS. For 50 vol.% AgPS, corresponding to 3.4 vol.% silver, the thermal conductivity was 2.03 ± 0.21 W m-1 K-1. The results show that the thermal conductivity is strongly correlated with the AgPS volume fraction, while maintaining a volume fraction of silver far below the commercial silver paste, which has typical filler fractions of 40 vol.% silver. The results of this work were compared to thermal measurements of the same material by other techniques, and advantages and disadvantages of the methods were finally discussed. © 2022 Author(s).
ISBN:00218979 (ISSN)
DOI:10.1063/5.0080682