Ultrafast carrier interactions in metal-halide perovskites probed with two-dimensional electronic spectroscopy

We use 2D electronic spectroscopy with sub-10-fs resolution to probe carrier-carrier scattering in perovskites. We report excitation-density dependent thermalization times below 100-fs. Strong coupling with excitonic states further reveals sub-bandgap states with low oscillator strength.

Bibliographic Details
Main Authors: Johannes M. Richter, Branchi Federico, Franco V. A. Camargo, Nagahara Tetsuhiko, Zhao Baodan, Richard H. Friend, Cerullo Giulio, Deschler Felix
Format: Article
Language:English
Published: EDP Sciences 2019-01-01
Series:EPJ Web of Conferences
Online Access:https://www.epj-conferences.org/articles/epjconf/pdf/2019/10/epjconf_up2019_04012.pdf