Rapid multiple-quantum three-dimensional fluorescence spectroscopy disentangles quantum pathways

Multidimensional spectroscopic tools are important to explore the details of molecular dynamics. Here the authors use shaped pulses to demonstrate a 3D fluorescence spectroscopy method to extract the fourth and higher-order nonlinear responses in light-molecule interaction.

Bibliographic Details
Main Authors: Stefan Mueller, Julian Lüttig, Pavel Malý, Lei Ji, Jie Han, Michael Moos, Todd B. Marder, Uwe H. F. Bunz, Andreas Dreuw, Christoph Lambert, Tobias Brixner
Format: Article
Language:English
Published: Nature Publishing Group 2019-10-01
Series:Nature Communications
Online Access:https://doi.org/10.1038/s41467-019-12602-x