Insight into dynamic and steady-state active sites for nitrogen activation to ammonia by cobalt-based catalyst

The industrial synthesis of ammonia using iron-based Haber-Bosch catalyst requires harsh reaction conditions. Here the authors show co-existence of dynamic and steady-state single atom active sites over Co-N-C catalyst to facilitate nitrogen activation for ammonia synthesis under mild conditions.

Bibliographic Details
Main Authors: Xiuyun Wang, Xuanbei Peng, Wei Chen, Guangyong Liu, Anmin Zheng, Lirong Zheng, Jun Ni, Chak-tong Au, Lilong Jiang
Format: Article
Language:English
Published: Nature Publishing Group 2020-01-01
Series:Nature Communications
Online Access:https://doi.org/10.1038/s41467-020-14287-z