Quantifying redox-induced Schottky barrier variations in memristive devices via in operando spectromicroscopy with graphene electrodes

Resistive switching in metal oxides is related to the migration of donor defects. Here Baeumer et al. use in operandoX-ray spectromicroscopy to quantify the doping locally and show that small local variations in the donor concentration result in large variations in the device resistance.

Bibliographic Details
Main Authors: Christoph Baeumer, Christoph Schmitz, Astrid Marchewka, David N. Mueller, Richard Valenta, Johanna Hackl, Nicolas Raab, Steven P. Rogers, M. Imtiaz Khan, Slavomir Nemsak, Moonsub Shim, Stephan Menzel, Claus Michael Schneider, Rainer Waser, Regina Dittmann
Format: Article
Language:English
Published: Nature Publishing Group 2016-08-01
Series:Nature Communications
Online Access:https://doi.org/10.1038/ncomms12398
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spelling doaj-bf6c3f4cacb943e7929d9dfd86966d522021-05-11T11:02:33ZengNature Publishing GroupNature Communications2041-17232016-08-01711710.1038/ncomms12398Quantifying redox-induced Schottky barrier variations in memristive devices via in operando spectromicroscopy with graphene electrodesChristoph Baeumer0Christoph Schmitz1Astrid Marchewka2David N. Mueller3Richard Valenta4Johanna Hackl5Nicolas Raab6Steven P. Rogers7M. Imtiaz Khan8Slavomir Nemsak9Moonsub Shim10Stephan Menzel11Claus Michael Schneider12Rainer Waser13Regina Dittmann14Peter Gruenberg Institute, Forschungszentrum Juelich GmbH and JARA-FITPeter Gruenberg Institute, Forschungszentrum Juelich GmbH and JARA-FITInstitute of Materials in Electrical Engineering and Information Technology II, RWTH Aachen UniversityPeter Gruenberg Institute, Forschungszentrum Juelich GmbH and JARA-FITPeter Gruenberg Institute, Forschungszentrum Juelich GmbH and JARA-FITPeter Gruenberg Institute, Forschungszentrum Juelich GmbH and JARA-FITPeter Gruenberg Institute, Forschungszentrum Juelich GmbH and JARA-FITDepartment of Materials Science and Engineering and Materials Research Laboratory, University of IllinoisPeter Gruenberg Institute, Forschungszentrum Juelich GmbH and JARA-FITPeter Gruenberg Institute, Forschungszentrum Juelich GmbH and JARA-FITDepartment of Materials Science and Engineering and Materials Research Laboratory, University of IllinoisPeter Gruenberg Institute, Forschungszentrum Juelich GmbH and JARA-FITPeter Gruenberg Institute, Forschungszentrum Juelich GmbH and JARA-FITPeter Gruenberg Institute, Forschungszentrum Juelich GmbH and JARA-FITPeter Gruenberg Institute, Forschungszentrum Juelich GmbH and JARA-FITResistive switching in metal oxides is related to the migration of donor defects. Here Baeumer et al. use in operandoX-ray spectromicroscopy to quantify the doping locally and show that small local variations in the donor concentration result in large variations in the device resistance.https://doi.org/10.1038/ncomms12398
collection DOAJ
language English
format Article
sources DOAJ
author Christoph Baeumer
Christoph Schmitz
Astrid Marchewka
David N. Mueller
Richard Valenta
Johanna Hackl
Nicolas Raab
Steven P. Rogers
M. Imtiaz Khan
Slavomir Nemsak
Moonsub Shim
Stephan Menzel
Claus Michael Schneider
Rainer Waser
Regina Dittmann
spellingShingle Christoph Baeumer
Christoph Schmitz
Astrid Marchewka
David N. Mueller
Richard Valenta
Johanna Hackl
Nicolas Raab
Steven P. Rogers
M. Imtiaz Khan
Slavomir Nemsak
Moonsub Shim
Stephan Menzel
Claus Michael Schneider
Rainer Waser
Regina Dittmann
Quantifying redox-induced Schottky barrier variations in memristive devices via in operando spectromicroscopy with graphene electrodes
Nature Communications
author_facet Christoph Baeumer
Christoph Schmitz
Astrid Marchewka
David N. Mueller
Richard Valenta
Johanna Hackl
Nicolas Raab
Steven P. Rogers
M. Imtiaz Khan
Slavomir Nemsak
Moonsub Shim
Stephan Menzel
Claus Michael Schneider
Rainer Waser
Regina Dittmann
author_sort Christoph Baeumer
title Quantifying redox-induced Schottky barrier variations in memristive devices via in operando spectromicroscopy with graphene electrodes
title_short Quantifying redox-induced Schottky barrier variations in memristive devices via in operando spectromicroscopy with graphene electrodes
title_full Quantifying redox-induced Schottky barrier variations in memristive devices via in operando spectromicroscopy with graphene electrodes
title_fullStr Quantifying redox-induced Schottky barrier variations in memristive devices via in operando spectromicroscopy with graphene electrodes
title_full_unstemmed Quantifying redox-induced Schottky barrier variations in memristive devices via in operando spectromicroscopy with graphene electrodes
title_sort quantifying redox-induced schottky barrier variations in memristive devices via in operando spectromicroscopy with graphene electrodes
publisher Nature Publishing Group
series Nature Communications
issn 2041-1723
publishDate 2016-08-01
description Resistive switching in metal oxides is related to the migration of donor defects. Here Baeumer et al. use in operandoX-ray spectromicroscopy to quantify the doping locally and show that small local variations in the donor concentration result in large variations in the device resistance.
url https://doi.org/10.1038/ncomms12398
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