Preparation of high orbital angular momentum Rydberg states by optical-millimeter-wave STIRAP

Rydberg states of molecules are intrinsically challenging to study due to the presence of fast non-radiative decay pathways, such as predissociation. However, selectively exciting Rydberg states with values of the orbital angular momentum (ℓ) ℓ ≳ 3 is a productive strategy to minimize this rapid dec...

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Bibliographic Details
Main Authors: Barnum, Timothy James (Author), Herburger, H. (Author), Grimes, David Darrah (Author), Jiang, Jun (Author), Field, Robert W (Author)
Other Authors: Massachusetts Institute of Technology. Department of Chemistry (Contributor)
Format: Article
Language:English
Published: AIP Publishing, 2020-10-26T14:39:59Z.
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