Shortcut to Self-Consistent Light-Matter Interaction and Realistic Spectra from First Principles
We introduce a simple approach to how an electromagnetic environment can be efficiently embedded into state-of-the-art electronic structure methods, taking the form of radiation-reaction forces. We demonstrate that this self-consistently provides access to radiative emission, natural linewidth, Lamb...
| Main Authors: | , |
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| Format: | Article |
| Language: | English |
| Published: |
American Physical Society
2022
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| Subjects: | |
| Online Access: | View Fulltext in Publisher |