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10.1103-PhysRevLett.128.156402 |
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|a 00319007 (ISSN)
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|a Shortcut to Self-Consistent Light-Matter Interaction and Realistic Spectra from First Principles
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|b American Physical Society
|c 2022
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|z View Fulltext in Publisher
|u https://doi.org/10.1103/PhysRevLett.128.156402
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|a We introduce a simple approach to how an electromagnetic environment can be efficiently embedded into state-of-the-art electronic structure methods, taking the form of radiation-reaction forces. We demonstrate that this self-consistently provides access to radiative emission, natural linewidth, Lamb shifts, strong coupling, electromagnetically induced transparency, Purcell-enhanced and superradiant emission. As an example, we illustrate its seamless integration into time-dependent density-functional theory with virtually no additional cost, presenting a convenient shortcut to light-matter interactions. © 2022 authors. Published by the American Physical Society.
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|a Chemical bonds
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|a Density functional theory
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|a Electromagnetic environments
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|a Electronic structure
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|a Electronic.structure
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|a First principles
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|a Light-matter interactions
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|a Radiation reactions
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|a Radiative emissions
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|a Reaction forces
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|a Simple approach
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|a Spectra's
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|a State of the art
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|a Johansson, G.
|e author
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|a Schäfer, C.
|e author
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|t Physical Review Letters
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